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二十面体1/1准晶中均匀刺猬序的磁动力学和非互易激发

Magnetic dynamics and nonreciprocal excitation in uniform hedgehog order in icosahedral 1/1 approximant crystal.

作者信息

Watanabe Shinji

机构信息

Department of Basic Sciences, Kyushu Institute of Technology, Kitakyushu, Fukuoka, 804-8550, Japan.

出版信息

Sci Rep. 2023 Sep 2;13(1):14438. doi: 10.1038/s41598-023-41292-1.

Abstract

The hedgehog state in the icosahedral quasicrystal (QC) has attracted great interest as the theoretical discovery of topological magnetic texture in aperiodic systems. The revealed magnetic dynamics exhibits nonreciprocal excitation in the vast extent of the reciprocal lattice [Formula: see text]-energy [Formula: see text] space, whose emergence mechanism remains unresolved. Here, we analyze the dynamical as well as static structure of the hedgehog order in the 1/1 approximant crystal (AC) composed of the cubic lattice with spatial inversion symmetry. We find that the dispersion of the magnetic excitation energy exhibits nonreciprocal feature along the N-P-[Formula: see text] line in the [Formula: see text] space. The dynamical structure factor exhibits highly structured intensities where high intensities appear in the high-energy branches along the [Formula: see text]-H line and the P-[Formula: see text]-N line in the [Formula: see text] space. The nonreciprocity in the 1/1 AC and also in the QC is understood to be ascribed to inversion symmetry breaking by the hedgehog ordering. The sharp contrast on the emergence regime of nonreciprocal magnetic excitation between the QC and the 1/1 AC indicates that the emergence in the vast [Formula: see text]-[Formula: see text] regime in the QC is attributed to the QC lattice structure.

摘要

二十面体准晶体(QC)中的刺猬态作为非周期系统中拓扑磁结构的理论发现引起了极大兴趣。所揭示的磁动力学在倒易晶格[公式:见正文]-能量[公式:见正文]空间的广阔范围内表现出非互易激发,其出现机制仍未得到解决。在此,我们分析了由具有空间反演对称性的立方晶格组成的1/1近似晶体(AC)中刺猬序的动力学以及静态结构。我们发现,磁激发能量的色散在[公式:见正文]空间中沿N - P - [公式:见正文]线表现出非互易特征。动态结构因子表现出高度结构化的强度,其中高强度出现在[公式:见正文]空间中沿[公式:见正文]-H线和P - [公式:见正文]-N线的高能分支中。1/1 AC以及QC中的非互易性被认为归因于刺猬序导致的反演对称性破缺。QC和1/1 AC之间非互易磁激发出现区域的鲜明对比表明,QC中在广阔的[公式:见正文]-[公式:见正文]区域中的出现归因于QC晶格结构。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/944c/10475090/4040ff3e7d5c/41598_2023_41292_Fig1_HTML.jpg

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