Bluschke Martin, Gupta Naman K, Jang Hoyoung, Husain Ali A, Lee Byungjune, Kim Minjune, Na MengXing, Dos Remedios Brandon, Smit Steef, Moen Peter, Park Sang-Youn, Kim Minseok, Jang Dogeun, Choi Hyeongi, Sutarto Ronny, Reid Alexander H, Dakovski Georgi L, Coslovich Giacomo, Nguyen Quynh L, Burdet Nicolas G, Lin Ming-Fu, Revcolevschi Alexandre, Park Jae-Hoon, Geck Jochen, Turner Joshua J, Damascelli Andrea, Hawthorn David G
Quantum Matter Institute, University of British Columbia, Vancouver, BC V6T 1Z4, Canada.
Department of Physics and Astronomy, University of British Columbia, Vancouver, BC V6T 1Z1, Canada.
Proc Natl Acad Sci U S A. 2024 Jun 4;121(23):e2400727121. doi: 10.1073/pnas.2400727121. Epub 2024 May 31.
Understanding the interplay between charge, nematic, and structural ordering tendencies in cuprate superconductors is critical to unraveling their complex phase diagram. Using pump-probe time-resolved resonant X-ray scattering on the (0 0 1) Bragg peak at the Cu [Formula: see text] and O [Formula: see text] resonances, we investigate nonequilibrium dynamics of [Formula: see text] nematic order and its association with both charge density wave (CDW) order and lattice dynamics in La[Formula: see text]Eu[Formula: see text]Sr[Formula: see text]CuO[Formula: see text]. The orbital selectivity of the resonant X-ray scattering cross-section allows nematicity dynamics associated with the planar O 2[Formula: see text] and Cu 3[Formula: see text] states to be distinguished from the response of anisotropic lattice distortions. A direct time-domain comparison of CDW translational-symmetry breaking and nematic rotational-symmetry breaking reveals that these broken symmetries remain closely linked in the photoexcited state, consistent with the stability of CDW topological defects in the investigated pump fluence regime.
理解铜酸盐超导体中电荷、向列相和结构有序倾向之间的相互作用对于揭示其复杂的相图至关重要。利用在铜([化学式:见原文])和氧([化学式:见原文])共振处对(0 0 1)布拉格峰进行泵浦-探测时间分辨共振X射线散射,我们研究了La[化学式:见原文]Eu[化学式:见原文]Sr[化学式:见原文]CuO[化学式:见原文]中[化学式:见原文]向列相序的非平衡动力学及其与电荷密度波(CDW)序和晶格动力学的关联。共振X射线散射截面的轨道选择性使得与平面O 2[化学式:见原文]和Cu 3[化学式:见原文]态相关的向列相动力学能够与各向异性晶格畸变的响应区分开来。对CDW平移对称性破缺和向列相旋转对称性破缺的直接时域比较表明,在光激发态下这些破缺的对称性仍然紧密相连,这与所研究的泵浦通量 regime 中CDW拓扑缺陷的稳定性一致。