Magdaleno Alvaro J, Cutler Mercy M, Suurmond Jesse J, Meléndez Marc, Delgado-Buscalioni Rafael, Seitz Michael, Prins Ferry
Condensed Matter Physics Center (IFIMAC) and Department of Condensed Matter Physics, Universidad Autónoma de Madrid, 28049 Madrid, Spain.
Condensed Matter Physics Center (IFIMAC) and Department of Theoretical Condensed Matter Physics, Universidad Autónoma de Madrid, 28049 Madrid, Spain.
Nanoscale. 2023 Sep 21;15(36):14831-14836. doi: 10.1039/d3nr03587e.
Transient Photoluminescence Microscopy (TPLM) allows for the direct visualization of carrier transport in semiconductor materials with sub nanosecond and few nanometer resolution. The technique is based on measuring changes in the spatial distribution of a diffraction limited population of carriers using spatiotemporal detection of the radiative decay of the carriers. The spatial resolution of TPLM is therefore primarily determined by the signal-to-noise-ratio (SNR). Here we present a method using cylindrical lenses to boost the signal acquisition in TPLM experiments. The resulting asymmetric magnification of the photoluminescence emission of the diffraction limited spot can increase the collection efficiency by more than a factor of 10, significantly reducing acquisition times and further boosting spatial resolution.
瞬态光致发光显微镜(TPLM)能够以亚纳秒和几纳米的分辨率直接观察半导体材料中的载流子传输。该技术基于通过对载流子辐射衰减的时空检测来测量衍射受限载流子群体空间分布的变化。因此,TPLM的空间分辨率主要由信噪比(SNR)决定。在此,我们提出一种在TPLM实验中使用柱面透镜来增强信号采集的方法。衍射受限光斑的光致发光发射所产生的不对称放大能够将收集效率提高10倍以上,显著减少采集时间并进一步提高空间分辨率。