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蓝色有机发光二极管的现状与挑战：综述

Status and Challenges of Blue OLEDs: A Review.

作者信息

Siddiqui Iram, Kumar Sudhir, Tsai Yi-Fang, Gautam Prakalp, Kesavan Kiran, Lin Jin-Ting, Khai Luke, Chou Kuo-Hsien, Choudhury Abhijeet, Grigalevicius Saulius, Jou Jwo-Huei

机构信息

Department of Materials Science and Engineering, National Tsing Hua University, Hsinchu 30013, Taiwan.

Institute for Chemical and Bioengineering, ETH Zürich, 8093 Zürich, Switzerland.

出版信息

Nanomaterials (Basel). 2023 Sep 8;13(18):2521. doi: 10.3390/nano13182521.

DOI:10.3390/nano13182521
PMID:37764550
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC10536903/
Abstract

Organic light-emitting diodes (OLEDs) have outperformed conventional display technologies in smartphones, smartwatches, tablets, and televisions while gradually growing to cover a sizable fraction of the solid-state lighting industry. Blue emission is a crucial chromatic component for realizing high-quality red, green, blue, and yellow (RGBY) and RGB white display technologies and solid-state lighting sources. For consumer products with desirable lifetimes and efficiency, deep blue emissions with much higher power efficiency and operation time are necessary prerequisites. This article reviews over 700 papers covering various factors, namely, the crucial role of blue emission for full-color displays and solid-state lighting, the performance status of blue OLEDs, and the systematic development of fluorescent, phosphorescent, and thermally activated delayed fluorescence blue emitters. In addition, various challenges concerning deep blue efficiency, lifetime, and approaches to realizing deeper blue emission and higher efficacy for blue OLED devices are also described.

摘要

有机发光二极管（OLED）在智能手机、智能手表、平板电脑和电视领域的表现已超越传统显示技术，同时逐渐在固态照明行业占据了相当大的份额。蓝光发射是实现高质量红、绿、蓝、黄（RGBY）和RGB白色显示技术以及固态照明光源的关键色彩成分。对于具有理想寿命和效率的消费产品而言，具备更高功率效率和运行时间的深蓝色发射是必要前提。本文综述了700多篇论文，涵盖了各种因素，即蓝光发射在全彩显示和固态照明中的关键作用、蓝色OLED的性能状况，以及荧光、磷光和热激活延迟荧光蓝色发光体的系统开发。此外，还描述了与深蓝色效率、寿命相关的各种挑战，以及实现蓝色OLED器件更深蓝色发射和更高效率的方法。

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Polymers (Basel). 2024 Aug 20;16(16):2347. doi: 10.3390/polym16162347.
9
The First Example of the Friedel-Crafts Cyclization Leading to (10-Hydroxy-9,10-dihydroanthr-9-yl)phosphonium Salts without the Expected Bradsher Dehydration.首次报道 Friedel-Crafts 环化反应得到（10-羟基-9,10-二氢蒽-9-基）磷翁盐，而没有预期的 Bradsher 脱水。
Int J Mol Sci. 2024 Feb 1;25(3):1741. doi: 10.3390/ijms25031741.
高效蜡烛光有机发光二极管，具有极低的色温。
Molecules. 2021 Dec 13;26(24):7558. doi: 10.3390/molecules26247558.
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Long-lived spin-polarized intermolecular exciplex states in thermally activated delayed fluorescence-based organic light-emitting diodes.基于热激活延迟荧光的有机发光二极管中的长寿命自旋极化分子间激基复合物态。
Sci Adv. 2021 Nov 19;7(47):eabj9961. doi: 10.1126/sciadv.abj9961. Epub 2021 Nov 17.
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Room-Temperature Phosphorescence and Thermally Activated Delayed Fluorescence in the Pd Complex: Mechanism and Dual Upconversion Channels.室温磷光和 Pd 配合物中的热激活延迟荧光：机理和双重上转换通道。
J Phys Chem Lett. 2021 Jul 1;12(25):5944-5950. doi: 10.1021/acs.jpclett.1c01558. Epub 2021 Jun 22.
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Improved Efficiency and Lifetime of Deep-Blue Hyperfluorescent Organic Light-Emitting Diode using Pt(II) Complex as Phosphorescent Sensitizer.使用Pt(II)配合物作为磷光敏化剂提高深蓝色超荧光有机发光二极管的效率和寿命。
Adv Sci (Weinh). 2021 Aug;8(16):e2100586. doi: 10.1002/advs.202100586. Epub 2021 Jun 16.
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Solution-Processed OLEDs Based on Thermally Activated Delayed Fluorescence Copper(I) Complexes with Intraligand Charge-Transfer Excited State.基于热激活延迟荧光铜（I）配合物的溶液处理 OLED，其激发态为配体内电荷转移态。
Molecules. 2021 Feb 20;26(4):1125. doi: 10.3390/molecules26041125.
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Harvesting triplet excitons for near-infrared electroluminescence via thermally activated delayed fluorescence channel.通过热激活延迟荧光通道收集用于近红外电致发光的三重态激子。
iScience. 2021 Feb 3;24(2):102123. doi: 10.1016/j.isci.2021.102123. eCollection 2021 Feb 19.
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Approaches for Long Lifetime Organic Light Emitting Diodes.长寿命有机发光二极管的方法。
Adv Sci (Weinh). 2020 Nov 12;8(1):2002254. doi: 10.1002/advs.202002254. eCollection 2020 Jan.
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Highly Efficient Deep-Blue OLEDs using a TADF Emitter with a Narrow Emission Spectrum and High Horizontal Emitting Dipole Ratio.使用具有窄发射光谱和高横向发射偶极比的热活化延迟荧光（TADF）发射体的高效深蓝色有机发光二极管
Adv Mater. 2020 Nov;32(47):e2004083. doi: 10.1002/adma.202004083. Epub 2020 Oct 20.