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记忆诱导的胶体哑铃排列

Memory-induced alignment of colloidal dumbbells.

作者信息

Krishna Kumar Karthika, Caspers Juliana, Ginot Félix, Krüger Matthias, Bechinger Clemens

机构信息

Fachbereich Physik, Universität Konstanz, Konstanz, 78457, Germany.

Institute for Theoretical Physics, Georg-August-Universität Göttingen, Göttingen, 37073, Germany.

出版信息

Sci Rep. 2023 Oct 13;13(1):17409. doi: 10.1038/s41598-023-44547-z.

Abstract

When a colloidal probe is forced through a viscoelastic fluid which is characterized by a long stress-relaxation time, the fluid is excited out of equilibrium. This is leading to a number of interesting effects including a non-trivial recoil of the probe when the driving force is removed. Here, we experimentally and theoretically investigate the transient recoil dynamics of non-spherical particles, i.e., colloidal dumbbells. In addition to a translational recoil of the dumbbells, we also find a pronounced angular reorientation which results from the relaxation of the surrounding fluid. Our findings are in good agreement with a Langevin description based on the symmetries of a director (dumbbell) as well as a microscopic bath-rod model. Remarkably, we find an instability with amplified fluctuations when the dumbbell is oriented perpendicular to the direction of driving. Our results demonstrate the complex behavior of non-spherical objects within a relaxing environment which are of immediate interest for the motion of externally but also self-driven asymmetric objects in viscoelastic fluids.

摘要

当一个胶体探针被迫穿过一种具有长应力松弛时间特征的粘弹性流体时,流体被激发至非平衡状态。这会导致许多有趣的效应,包括在驱动力移除时探针出现非平凡的反冲。在此,我们通过实验和理论研究非球形颗粒,即胶体哑铃的瞬态反冲动力学。除了哑铃的平动反冲外,我们还发现由于周围流体的松弛而导致的明显角重新定向。我们的发现与基于指向矢(哑铃)对称性的朗之万描述以及微观浴棒模型高度吻合。值得注意的是,当哑铃垂直于驱动方向取向时,我们发现了波动放大的不稳定性。我们的结果展示了在松弛环境中非球形物体的复杂行为,这对于粘弹性流体中外加驱动以及自驱动不对称物体的运动具有直接意义。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/b9f7/10575873/640371a419da/41598_2023_44547_Fig1_HTML.jpg

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