Wu Xiaolong, Xu Yuanwu, Peng Jingxuan, Xia Zhiping, Kupecki Jakub, Li Xi
Shenzhen Huazhong University of Science and Technology Research Institute, Shenzhen 518055, P. R. China.
Belt and Road Joint Laboratory on Measurement and Control Technology, School of Artificial Intelligence and Automation, Huazhong University of Science and Technology, Wuhan 430074, P. R. China.
ACS Omega. 2023 Sep 27;8(40):36876-36892. doi: 10.1021/acsomega.3c03928. eCollection 2023 Oct 10.
Steam reforming solid oxide fuel cell (SOFC) systems are important devices to promote carbon neutralization and clean energy conversion. It is difficult to monitor system working conditions in real time due to the possible fusion fault degradation under high temperatures and the seal environment, so it is necessary to design an effective system multifault degradation assessment strategy for solid oxide fuel cell systems. Therefore, in this paper, a novel hybrid model is developed. The hybrid model is built to look for the system fault reason based on first principles, machine learning (radial basis function neural network), and a multimodal classification algorithm. Then, stack, key balance of plant components (afterburner, heat exchanger, and reformer), thermoelectric performance, and system efficiency are studied during the progress of the system experiment. The results show that the novel hybrid model can track well the system operation trend, and solid oxide fuel cell system working dynamic performance can be obtained. Furthermore, four fault types of solid oxide fuel cell systems are analyzed with thermoelectric parameters and energy conversion efficiency based on transition and fault stages, and two cases are also successful by using the built model to decouple the multifault degradation fusion. In addition, the solid oxide fuel cell multifault degradation fusion assessment method proposed in this paper can also be used in other fuel cell systems.
蒸汽重整固体氧化物燃料电池(SOFC)系统是促进碳中和和清洁能源转换的重要装置。由于在高温和密封环境下可能出现熔合故障退化,实时监测系统工作状态较为困难,因此有必要为固体氧化物燃料电池系统设计一种有效的系统多故障退化评估策略。为此,本文开发了一种新型混合模型。该混合模型基于第一原理、机器学习(径向基函数神经网络)和多模态分类算法构建,用于寻找系统故障原因。然后,在系统实验过程中研究了电池堆、关键平衡部件(后燃器、热交换器和重整器)、热电性能和系统效率。结果表明,新型混合模型能够很好地跟踪系统运行趋势,并可获得固体氧化物燃料电池系统的工作动态性能。此外,基于过渡和故障阶段,利用热电参数和能量转换效率分析了固体氧化物燃料电池系统的四种故障类型,通过所构建的模型对多故障退化融合进行解耦的两个案例也取得了成功。此外,本文提出的固体氧化物燃料电池多故障退化融合评估方法也可应用于其他燃料电池系统。