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阳极支撑型固体氧化物燃料电池的性能分析:一种机器学习方法。

Performance Analysis of Anode-Supported Solid Oxide Fuel Cells: A Machine Learning Approach.

作者信息

Golbabaei Mohammad Hossein, Saeidi Varnoosfaderani Mohammadreza, Zare Arsalan, Salari Hirad, Hemmati Farshid, Abdoli Hamid, Hamawandi Bejan

机构信息

School of Metallurgy and Materials, College of Engineering, University of Tehran, Tehran 1417935840, Iran.

School of Metallurgy and Materials Engineering, Iran University of Science and Technology, Tehran 1684613114, Iran.

出版信息

Materials (Basel). 2022 Nov 3;15(21):7760. doi: 10.3390/ma15217760.

Abstract

Prior to the long-term utilization of solid oxide fuel cell (SOFC), one of the most remarkable electrochemical energy conversion devices, a variety of difficult experimental validation procedures is required, so it would be time-consuming and steep to predict the applicability of these devices in the future. For numerous years, extensive efforts have been made to develop mathematical models to predict the effects of various characteristics of solid oxide fuel cells (SOFCs) components on their performance (e.g., voltage). Taking advantage of the machine learning (ML) method, however, some issues caused by assumptions and calculation costs in mathematical modeling could be alleviated. This paper presents a machine learning approach to predict the anode-supported SOFCs performance as one of the most promising types of SOFCs based on architectural and operational variables. Accordingly, a dataset was collected from a study about the effects of cell parameters on the output voltage of a Ni-YSZ anode-supported cell. Convolutional machine learning models and multilayer perceptron neural networks were implemented to predict the current-voltage dependency. The resulting neural network model could properly predict, with more than 0.998 R score, a mean squared error of 9.6 × 10, and mean absolute error of 6 × 10 (V). Conventional models such as the Gaussian process as one of the most powerful models exhibits a prediction accuracy of 0.996 R score, 10 mean squared, and 6 × 10 (V) absolute error. The results showed that the built neural network could predict the effect of cell parameters on current-voltage dependency more accurately than previous mathematical and artificial neural network models. It is noteworthy that this procedure used in this study is general and can be easily applied to other materials datasets.

摘要

在长期使用固体氧化物燃料电池(SOFC)(最卓越的电化学能量转换装置之一)之前,需要进行各种困难的实验验证程序,因此预测这些装置未来的适用性既耗时又艰巨。多年来,人们付出了巨大努力来开发数学模型,以预测固体氧化物燃料电池(SOFC)组件的各种特性对其性能(例如电压)的影响。然而,利用机器学习(ML)方法,可以缓解数学建模中由假设和计算成本引起的一些问题。本文提出了一种机器学习方法,基于结构和运行变量来预测作为最有前景的SOFC类型之一的阳极支撑SOFC的性能。相应地,从一项关于电池参数对Ni-YSZ阳极支撑电池输出电压影响的研究中收集了一个数据集。实施了卷积机器学习模型和多层感知器神经网络来预测电流-电压依赖性。所得的神经网络模型能够以超过0.998的R分数、9.6×10的均方误差和6×10(V)的平均绝对误差进行准确预测。诸如高斯过程等传统模型作为最强大的模型之一,其预测准确率为0.996的R分数、10的均方误差和6×10(V)的绝对误差。结果表明,所构建的神经网络能够比先前的数学模型和人工神经网络模型更准确地预测电池参数对电流-电压依赖性的影响。值得注意的是,本研究中使用的这个程序具有通用性,并且可以很容易地应用于其他材料数据集。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7705/9655730/db37557268e8/materials-15-07760-g001.jpg

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