Fan Yihang, Xue Xiaotian, Yang Fei, Zhao Jianqiao, Xiong Xiaoyu, Sun Jingbo, Wang Weipeng, Shi Ji, Zhou Ji, Zhang Zhengjun
Key Laboratory of Advanced Materials (MOE), School of Materials Science and Engineering, Tsinghua University, Beijing 10084, People's Republic of China.
State Key Laboratory of New Ceramics and Fine Processing, School of Materials Science and Engineering, Tsinghua University, Beijing 100084, People's Republic of China.
Nano Lett. 2023 Nov 8;23(21):9900-9906. doi: 10.1021/acs.nanolett.3c02833. Epub 2023 Oct 20.
Scanning near-field optical microscope (SNOM) with nanoscale spatial resolution has been a powerful tool in studying the plasmonic properties of nano materials/structures. However, the quantification of the SNOM measurement remains a major challenge in the field due to the lack of reliable methodologies. We employed the point-dipole model to describe the tip-surface interaction upon laser illumination and theoretically derived the quantitative relationship between the measured results and the actual near-field electric field strength. Thus, we can experimentally reconstruct the near-field electric field through this theoretically calculated relationship. We also developed an experimental technique together with FEM simulation to get the above relationship experimentally and reconstruct the near-field electric field from the measurement by SNOM.
具有纳米级空间分辨率的扫描近场光学显微镜(SNOM)一直是研究纳米材料/结构等离子体特性的有力工具。然而,由于缺乏可靠的方法,SNOM测量的量化仍然是该领域的一个主要挑战。我们采用点偶极子模型来描述激光照射下的针尖-表面相互作用,并从理论上推导了测量结果与实际近场电场强度之间的定量关系。因此,我们可以通过这种理论计算的关系实验性地重建近场电场。我们还开发了一种实验技术,并结合有限元模拟,通过实验得到上述关系,并从SNOM测量中重建近场电场。