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SrTiO₃ 中的光致负微分电阻和耿氏振荡

Photoinduced Negative Differential Resistivity and Gunn Oscillations in SrTiO3.

作者信息

Soleimany Mehrzad, Alexe Marin

机构信息

Department of Physics, University of Warwick, Gibbet Hill Road, Coventry, CV4 7AL, UK.

Department of Materials and Earth Sciences, Technical University of Darmstadt, 64287, Darmstadt, Germany.

出版信息

Adv Sci (Weinh). 2023 Dec;10(35):e2306420. doi: 10.1002/advs.202306420. Epub 2023 Oct 23.

DOI:10.1002/advs.202306420
PMID:37870178
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC10724436/
Abstract

SrTiO , a perovskite oxide, holds significant potential for application in the field of oxide electronics. Notably, its photoelectric activity in the low temperature regime, which overlaps with the quantum paraelectric state, exhibits remarkable characteristics. In this study, it is demonstrated that when photo-excited with above band gap energy photons, SrTiO exhibits non-linear transport of photocarriers and voltage-controlled negative resistance, resulting from an intervalley transfer of photo-induced electrons. As a consequence of the negative resistance, the photocurrent becomes unstable and spontaneously gives rise to low frequency Gunn-like oscillations.

摘要

钛酸锶(SrTiO₃)是一种钙钛矿氧化物,在氧化物电子学领域具有巨大的应用潜力。值得注意的是,它在低温区域的光电活性与量子顺电态重叠,呈现出显著的特性。在本研究中,结果表明,当用高于带隙能量的光子进行光激发时,钛酸锶(SrTiO₃)会出现光载流子的非线性传输和压控负电阻,这是由光致电子的谷间转移引起的。由于负电阻的存在,光电流变得不稳定,并自发产生低频耿氏(Gunn)样振荡。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7eb8/10724436/155583be04c7/ADVS-10-2306420-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7eb8/10724436/e7a8d8848d93/ADVS-10-2306420-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7eb8/10724436/bc0abff39537/ADVS-10-2306420-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7eb8/10724436/155583be04c7/ADVS-10-2306420-g004.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7eb8/10724436/e7a8d8848d93/ADVS-10-2306420-g003.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7eb8/10724436/bc0abff39537/ADVS-10-2306420-g002.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/7eb8/10724436/155583be04c7/ADVS-10-2306420-g004.jpg

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本文引用的文献

1
Anomalous intense coherent secondary photoemission from a perovskite oxide.钙钛矿氧化物中的反常强相干二次光电子发射。
Nature. 2023 May;617(7961):493-498. doi: 10.1038/s41586-023-05900-4. Epub 2023 Mar 8.
2
Emergence of room-temperature ferroelectricity at reduced dimensions.在降低维度下室温铁电性的出现。
Science. 2015 Sep 18;349(6254):1314-7. doi: 10.1126/science.aaa6442.