Dos Santos Dias M, Biniskos N, Dos Santos F J, Schmalzl K, Persson J, Bourdarot F, Marzari N, Blügel S, Brückel T, Lounis S
Peter Grünberg Institut and Institute for Advanced Simulation, Forschungszentrum Jülich & JARA, D-52425, Jülich, Germany.
Faculty of Physics, University of Duisburg-Essen and CENIDE, D-47053, Duisburg, Germany.
Nat Commun. 2023 Nov 11;14(1):7321. doi: 10.1038/s41467-023-43042-3.
The phase of the quantum-mechanical wave function can encode a topological structure with wide-ranging physical consequences, such as anomalous transport effects and the existence of edge states robust against perturbations. While this has been exhaustively demonstrated for electrons, properties associated with the elementary quasiparticles in magnetic materials are still underexplored. Here, we show theoretically and via inelastic neutron scattering experiments that the bulk ferromagnet MnGe hosts gapped topological Dirac magnons. Although inversion symmetry prohibits a net Dzyaloshinskii-Moriya interaction in the unit cell, it is locally allowed and is responsible for the gap opening in the magnon spectrum. This gap is predicted and experimentally verified to close by rotating the magnetization away from the c-axis with an applied magnetic field. Hence, MnGe realizes a gapped Dirac magnon material in three dimensions. Its tunability by chemical doping or by thin film nanostructuring defines an exciting new platform to explore and design topological magnons. More generally, our experimental route to verify and control the topological character of the magnons is applicable to bulk centrosymmetric hexagonal materials, which calls for systematic investigation.
量子力学波函数的相位能够编码一种具有广泛物理效应的拓扑结构,诸如反常输运效应以及对微扰具有鲁棒性的边缘态的存在。虽然这已在电子方面得到详尽证明,但与磁性材料中的基本准粒子相关的性质仍未得到充分探索。在此,我们通过理论计算以及非弹性中子散射实验表明,体心铁磁体MnGe存在带隙的拓扑狄拉克磁振子。尽管空间反演对称性禁止在晶胞中存在净的Dzyaloshinskii-Moriya相互作用,但在局部是允许的,并且它是磁振子能谱中带隙打开的原因。通过施加磁场使磁化方向偏离c轴,预计并通过实验验证了这个带隙会关闭。因此,MnGe在三维空间中实现了一种带隙狄拉克磁振子材料。其通过化学掺杂或薄膜纳米结构实现的可调性定义了一个用于探索和设计拓扑磁振子的令人兴奋的新平台。更一般地说,我们验证和控制磁振子拓扑特性的实验途径适用于体心中心对称的六角材料,这需要进行系统研究。