Fu Yong, Wang Bincheng, Wang Kan, Tang Xiangyu, Li Baochang, Yin Zhiming, Han Jiaxin, Lin C D, Jin Cheng
Department of Applied Physics, Nanjing University of Science and Technology, Nanjing, Jiangsu 210094, China.
Department of Physics, James R. Macdonald Laboratory, Kansas State University, Manhattan, KS 66506.
Proc Natl Acad Sci U S A. 2024 Jan 9;121(2):e2307836121. doi: 10.1073/pnas.2307836121. Epub 2024 Jan 3.
High-harmonic generation from a gas target exhibits sharp spectral features and rapid phase variation near the Cooper minimum. By applying spectral filtering, shaped isolated attosecond pulses can be generated where the pulse is split into two in the time domain. Using such shaped extreme-ultraviolet (XUV) pulses, we theoretically study attosecond transient absorption (ATA) spectra of helium [Formula: see text] autoionizing state which is resonantly coupled to the [Formula: see text] dark state by a time-delayed infrared laser. Our simulations show that the asymmetric [Formula: see text] Fano line shape can be readily tuned into symmetric Lorentzian within the time delay of a few tens of attoseconds. Such efficient control is due to the destructive interference in the generation of the [Formula: see text] state when it is excited by a strongly shaped XUV pulse. This is to be compared to prior experiments where tuning the line shape of a Fano resonance would take tens of femtoseconds. We also show that the predicted ATA spectral line shape can be observed experimentally after propagation in a gas medium. Our results suggest that strongly shaped attosecond XUV pulses offer the opportunity for controlling and probing fine features of narrow resonances on the few-ten attoseconds timescale.
气体靶产生的高次谐波在库珀极小值附近呈现出尖锐的光谱特征和快速的相位变化。通过应用光谱滤波,可以产生整形的孤立阿秒脉冲,此时脉冲在时域中被分成两部分。利用这种整形的极紫外(XUV)脉冲,我们从理论上研究了氦的[公式:见正文]自电离态的阿秒瞬态吸收(ATA)光谱,该自电离态通过延迟红外激光与[公式:见正文]暗态发生共振耦合。我们的模拟表明,在几十阿秒的时间延迟内,不对称的[公式:见正文]法诺线形可以很容易地调制成对称的洛伦兹线形。这种高效的控制是由于当[公式:见正文]态由强整形的XUV脉冲激发时,在其产生过程中发生了相消干涉。这与之前将法诺共振的线形调谐需要几十飞秒的实验形成对比。我们还表明,预测的ATA光谱线形在气体介质中传播后可以通过实验观察到。我们的结果表明,强整形的阿秒XUV脉冲为在几十阿秒时间尺度上控制和探测窄共振的精细特征提供了机会。