Boltaev Ganjaboy S, Ganeev Rashid A, Alnaser Ali S
Opt Express. 2024 Jan 1;32(1):113-124. doi: 10.1364/OE.507586.
High repetition coherent extreme ultraviolet (XUV) harmonics offer a powerful tool for investigating electron dynamics and understanding the underlying physics in a wide range of systems. We demonstrate the utilization of combined three-color (ω+2ω+3ω) laser fields in the generation of coherent extreme ultraviolet radiation in mixed noble gases. The three-color field results from the combination of fundamental, second-, and third-order harmonics of the near-infrared laser pulses in the nonlinear crystals. Different noble gases were selected as gas targets based on their ionization potentials, which are important parameters for generating higher cut-offs and intensities for the XUV harmonics. Enhanced XUV harmonic intensities were observed in the mixture of He + Kr gases when using three-color laser fields, compared to harmonics generated in the He + Kr mixture under a single-color pump. On the other hand, suppression of XUV harmonic intensity was observed in the mixture of He + Xe under the three-color pump due to the highest ionization level for these two mixed gases at similar laser conditions. Strong harmonic yields in the range of 25 to 80 eV of photon energy were observed.
高重复率相干极紫外(XUV)谐波为研究电子动力学和理解广泛系统中的基础物理提供了一个强大工具。我们展示了利用组合三色(ω + 2ω + 3ω)激光场在混合稀有气体中产生相干极紫外辐射。三色场由近红外激光脉冲在非线性晶体中的基频、二次谐波和三次谐波组合而成。基于它们的电离势选择不同的稀有气体作为气体靶,电离势是产生更高截止频率和XUV谐波强度的重要参数。与在单色泵浦下He + Kr混合物中产生的谐波相比,当使用三色激光场时,在He + Kr气体混合物中观察到增强的XUV谐波强度。另一方面,由于在相似激光条件下这两种混合气体的电离水平最高,在三色泵浦下He + Xe混合物中观察到XUV谐波强度受到抑制。观察到在25至80 eV光子能量范围内有很强的谐波产率。