Fasolato Claudia, Stellino Elena, Principi Emiliano, Mincigrucci Riccardo, Pelli-Cresi Jacopo Stefano, Foglia Laura, Postorino Paolo, Sacchetti Francesco, Petrillo Caterina
Dipartimento di Fisica e Geologia, Università di Perugia, Perugia I-06123, Italy.
Istituto dei Sistemi Complessi, Consiglio Nazionale delle Ricerche (CNR-ISC), Roma I-00185, Italy.
Proc Natl Acad Sci U S A. 2024 Jan 23;121(4):e2221293121. doi: 10.1073/pnas.2221293121. Epub 2024 Jan 19.
We study the Thomson scattering from highly oriented pyrolitic graphite excited by the extreme ultraviolet, coherent pulses of FERMI free electron laser (FEL). An apparent nonlinear behavior is observed and fully described in terms of the coherent nature of both exciting FEL beam and scattered radiation, producing an intensity-dependent enhancement of the Thomson scattering cross-section. The process resembles Dicke's superradiant phenomenon and is thus interpreted as the observation of superradiant Thomson scattering. The process also triggers the creation of coherent, low- ([Formula: see text] 0.3 Å[Formula: see text]), low energy phonons. The experimental data and analysis provide quantitative information on the sample characteristics, absorption, scattering factor, and coherent phonon energies and populations and open the route for the investigation of the deep nature of complex materials.
我们研究了由费米自由电子激光(FEL)的极紫外相干脉冲激发的高度取向热解石墨中的汤姆逊散射。观察到一种明显的非线性行为,并根据激发FEL光束和散射辐射的相干性质进行了全面描述,从而产生了强度依赖的汤姆逊散射截面增强。该过程类似于狄克超辐射现象,因此被解释为超辐射汤姆逊散射的观测。该过程还触发了相干、低能量([公式:见正文]0.3 Å[公式:见正文])声子的产生。实验数据和分析提供了关于样品特性、吸收、散射因子以及相干声子能量和数量的定量信息,并为研究复杂材料的深层性质开辟了道路。