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特邀文章:使用具有可变偏振的种子自由电子激光脉冲的相干成像:初步结果与研究机遇

Invited article: Coherent imaging using seeded free-electron laser pulses with variable polarization: first results and research opportunities.

作者信息

Capotondi F, Pedersoli E, Mahne N, Menk R H, Passos G, Raimondi L, Svetina C, Sandrin G, Zangrando M, Kiskinova M, Bajt S, Barthelmess M, Fleckenstein H, Chapman H N, Schulz J, Bach J, Frömter R, Schleitzer S, Müller L, Gutt C, Grübel G

机构信息

FERMI, Elettra-Sincrotrone Trieste, SS 14 - km 163.5, 34149 Basovizza, Trieste, Italy.

出版信息

Rev Sci Instrum. 2013 May;84(5):051301. doi: 10.1063/1.4807157.

Abstract

FERMI@Elettra, the first vacuum ultraviolet and soft X-ray free-electron laser (FEL) using by default a "seeded" scheme, became operational in 2011 and has been opened to users since December 2012. The parameters of the seeded FERMI FEL pulses and, in particular, the superior control of emitted radiation in terms of spectral purity and stability meet the stringent requirements for single-shot and resonant coherent diffraction imaging (CDI) experiments. The advantages of the intense seeded FERMI pulses with variable polarization have been demonstrated with the first experiments performed using the multipurpose experimental station operated at the diffraction and projection imaging (DiProI) beamline. The results reported here were obtained with fixed non-periodic targets during the commissioning period in 2012 using 20-32 nm wavelength range. They demonstrate that the performance of the FERMI FEL source and the experimental station meets the requirements of CDI, holography, and resonant magnetic scattering in both multi- and single-shot modes. Moreover, we present the first magnetic scattering experiments employing the fully circularly polarized FERMI pulses. The ongoing developments aim at pushing the lateral resolution by using shorter wavelengths provided by double-stage cascaded FERMI FEL-2 and probing ultrafast dynamic processes using different pump-probe schemes, including jitter-free seed laser pump or FEL-pump∕FEL-probe with two color FEL pulses generated by the same electron bunch.

摘要

费米@埃莱特拉是首个默认采用“种子注入”方案的真空紫外和软X射线自由电子激光(FEL),于2011年投入运行,并自2012年12月起向用户开放。种子注入式费米自由电子激光脉冲的参数,特别是在光谱纯度和稳定性方面对发射辐射的卓越控制,满足了单次和共振相干衍射成像(CDI)实验的严格要求。利用在衍射与投影成像(DiProI)光束线运行的多用途实验站进行的首批实验,已证明了具有可变偏振的高强度种子注入式费米脉冲的优势。此处报告的结果是在2012年调试期间使用20 - 32纳米波长范围的固定非周期性靶材获得的。这些结果表明,费米自由电子激光源和实验站的性能在多次和单次模式下均满足CDI、全息术和共振磁散射的要求。此外,我们展示了首次采用完全圆偏振费米脉冲的磁散射实验。正在进行的研发旨在通过使用两级级联费米自由电子激光 - FEL - 2提供的更短波长来提高横向分辨率,并使用不同的泵浦 - 探测方案,包括无抖动种子激光泵浦或具有由同一电子束产生的双色自由电子激光脉冲的自由电子激光泵浦∕自由电子激光探测,来探测超快动态过程。

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