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格陵兰冰盖大量汞释放的说法被推翻。

Large mercury release from the Greenland Ice Sheet invalidated.

作者信息

Jørgensen Christian Juncher, Søndergaard Jens, Larsen Martin Mørk, Kjeldsen Kristian Kjellerup, Rosa Diogo, Sapper Sarah Elise, Heimbürger-Boavida Lars-Eric, Kohler Stephen G, Wang Feiyue, Gao Zhiyuan, Armstrong Debbie, Albers Christian Nyrop

机构信息

Department of Ecoscience, Aarhus University, Roskilde 4000, Denmark.

Geological Survey of Denmark and Greenland, Copenhagen 1350, Denmark.

出版信息

Sci Adv. 2024 Jan 26;10(4):eadi7760. doi: 10.1126/sciadv.adi7760.

DOI:10.1126/sciadv.adi7760
PMID:38277451
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC10816687/
Abstract

The major input of mercury (Hg) to the Arctic is normally ascribed to long-range transport of anthropogenic Hg emissions. Recently, alarming concentrations of Hg in meltwater from the Greenland Ice Sheet (GrIS) were reported with bedrock as the proposed source. Reported Hg concentrations were 100 to 1000 times higher than in known freshwater systems of Greenland, calling for independent validation of the extraordinary concentrations and conclusions. Here, we present measurements of Hg at 21 glacial outlets in West Greenland showing that extreme Hg concentrations cannot be reproduced. In contrast, we find that meltwater from below the GrIS is very low in Hg, has minor implications for the global Hg budget, and pose only a very limited risk for local communities and the natural environment of Greenland.

摘要

北极汞(Hg)的主要输入通常归因于人为汞排放的远距离传输。最近,有报道称格陵兰冰盖(GrIS)融水中汞浓度惊人,提出基岩为潜在来源。报告的汞浓度比格陵兰已知淡水系统中的浓度高100至1000倍,这就需要对这些异常浓度和结论进行独立验证。在此,我们展示了对西格陵兰21个冰川出水口汞的测量结果,表明无法再现极端汞浓度。相反,我们发现GrIS下方的融水汞含量极低,对全球汞预算影响较小,对格陵兰当地社区和自然环境仅构成非常有限的风险。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9d2f/10816687/279a9b725209/sciadv.adi7760-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9d2f/10816687/023cd25f9aa0/sciadv.adi7760-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9d2f/10816687/f5da6ce1cd5f/sciadv.adi7760-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9d2f/10816687/279a9b725209/sciadv.adi7760-f3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9d2f/10816687/023cd25f9aa0/sciadv.adi7760-f1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9d2f/10816687/f5da6ce1cd5f/sciadv.adi7760-f2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/9d2f/10816687/279a9b725209/sciadv.adi7760-f3.jpg

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本文引用的文献

1
Greenland melt drives continuous export of methane from the ice-sheet bed.格陵兰冰盖融化促使甲烷持续从冰盖底部排出。
Nature. 2019 Jan;565(7737):73-77. doi: 10.1038/s41586-018-0800-0. Epub 2019 Jan 2.
2
First observation of direct methane emission to the atmosphere from the subglacial domain of the Greenland Ice Sheet.首次观测到格陵兰冰盖冰下区域向大气直接排放甲烷。
Sci Rep. 2018 Nov 9;8(1):16623. doi: 10.1038/s41598-018-35054-7.
3
Shallow methylmercury production in the marginal sea ice zone of the central Arctic Ocean.
北冰洋中部边缘海冰区浅层甲基汞的生成
Sci Rep. 2015 May 20;5:10318. doi: 10.1038/srep10318.
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Mercury exports from a High-Arctic river basin in Northeast Greenland (74°N) largely controlled by glacial lake outburst floods.格陵兰岛东北部(74°N)高北极河流流域的汞出口主要受冰川湖溃决洪水控制。
Sci Total Environ. 2015 May 1;514:83-91. doi: 10.1016/j.scitotenv.2015.01.097. Epub 2015 Feb 6.
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Sci Total Environ. 2005 Jan 20;337(1-3):253-63. doi: 10.1016/j.scitotenv.2004.07.006.
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Mercury in dated Greenland marine sediments.格陵兰岛海洋沉积物年代测定中的汞含量
Sci Total Environ. 2000 Jan 17;245(1-3):61-72. doi: 10.1016/s0048-9697(99)00433-7.
7
Calculation of soil-water and benthic sediment partition coefficients for mercury.汞的土壤-水和底栖沉积物分配系数的计算。
Chemosphere. 1997 Aug;35(4):791-808. doi: 10.1016/s0045-6535(97)00200-2.
8
Mercury contamination of sea water samples stored in polyethylene containers.储存在聚乙烯容器中的海水样本的汞污染。
Anal Chem. 1975 Mar;47(3):592-5. doi: 10.1021/ac60353a012.