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通过河流进入海洋的陆源大塑料和微塑料的过程及输运通量。

The processes and transport fluxes of land-based macroplastics and microplastics entering the ocean via rivers.

作者信息

Wang Teng, Li Baojie, Shi Huahong, Ding Yongcheng, Chen Hongyu, Yuan Feng, Liu Rongze, Zou Xinqing

机构信息

Key Laboratory of Marine Hazards Forecasting, Ministry of Natural Resources, Hohai University, Nanjing 210024, China; Jiangsu Province Engineering Research Center for Marine Bio-resources Sustainable Utilization & Nanjing Outskirts Sea-Atmosphere Interface Field Scientific Observation Research Station & College of Oceanography, Hohai University, Nanjing 210024, China.

Collaborative Innovation Center of Atmospheric Environment and Equipment Technology, Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, School of Environmental Science and Engineering, Nanjing University of Information Science & Technology, Nanjing 210044, China.

出版信息

J Hazard Mater. 2024 Mar 15;466:133623. doi: 10.1016/j.jhazmat.2024.133623. Epub 2024 Jan 26.

Abstract

Approximately 80% of marine plastic waste originates from land-based sources and enters oceans through rivers. Hence, to create effective regulations, it is crucial to thoroughly examine the processes by which land-based plastic waste flows into marine environments. To this end, this review covers the complete journey of macro- and microplastics from their initial input into rivers to their ultimate release into oceans. Here, we also discuss the primary influencing factors and current popular research topics. Additionally, the principles, applicability, accuracy, uncertainty, and potential improvement of the standard methods used for flux estimation at each stage are outlined. Emission estimates of land-based macro- and microplastics are typically assessed using the emission factor approach, coefficient accounting approach, or material flow analysis. Accurately estimating mismanaged plastic waste is crucial for reducing uncertainty in the macroplastic emission inventory. In our review of the processes by which land-originating plastics enter rivers, we categorized them into two major types: point-source and diffuse-source pollution. Land surface hydrological models simulate transport from diffuse sources to rivers, necessitating further research. Riverine (micro)plastic flux to the ocean is often estimated using monitoring statistics and watershed hydrological models at the watershed scale; however, standardized monitoring methods have not yet been established. At the global scale, algorithms based on river datasets are often used, which require further improvements in river data selection and microplastic number-mass conversion factors. Furthermore, the article summarizes the accuracy and sources of uncertainty of various methods. Future research efforts should focus on quantifying and mitigating uncertainties in resultant projections. Overall, this review deepens our understanding of the processes by which land-based plastic waste enters the ocean and helps scholars efficiently select or improve relevant methods when studying land-ocean transport fluxes.

摘要

大约80%的海洋塑料垃圾源自陆地来源,并通过河流进入海洋。因此,要制定有效的法规,彻底研究陆地塑料垃圾流入海洋环境的过程至关重要。为此,本综述涵盖了宏观和微观塑料从最初进入河流到最终释放到海洋的完整过程。在此,我们还讨论了主要影响因素和当前热门的研究课题。此外,还概述了在每个阶段用于通量估算的标准方法的原理、适用性、准确性、不确定性和潜在改进。陆地宏观和微观塑料的排放估算通常采用排放因子法、系数核算法或物质流分析法。准确估算管理不善的塑料垃圾对于减少宏观塑料排放清单中的不确定性至关重要。在我们对源自陆地的塑料进入河流过程的综述中,我们将其分为两种主要类型:点源污染和非点源污染。陆地表面水文模型模拟了从非点源到河流的传输,这需要进一步研究。河流(微)塑料向海洋的通量通常在流域尺度上使用监测统计数据和流域水文模型进行估算;然而,尚未建立标准化的监测方法。在全球尺度上,通常使用基于河流数据集的算法,这需要在河流数据选择和微塑料数量-质量转换因子方面进一步改进。此外,本文总结了各种方法的准确性和不确定性来源。未来的研究工作应集中在量化和减轻结果预测中的不确定性。总体而言,本综述加深了我们对陆地塑料垃圾进入海洋过程的理解,并有助于学者在研究陆海传输通量时有效地选择或改进相关方法。

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