Chen Jingyu, Zhang Wenjie, Yang Wenzhi, Xi Fengcheng, He Hongyi, Liang Minghao, Dong Qian, Hou Jiawang, Wang Mengbin, Yu Guocan, Zhou Jiong
Department of Chemistry, College of Sciences, Northeastern University, Shenyang, 110819, PR China.
ZJU-Hangzhou Global Scientific and Technological Innovation Center, Zhejiang University, Hangzhou, 311215, PR China.
Nat Commun. 2024 Feb 10;15(1):1260. doi: 10.1038/s41467-024-45592-6.
The combination of macrocyclic chemistry with co-crystal engineering has promoted the development of materials with vapochromic behaviors in supramolecular science. Herein, we develop a macrocycle co-crystal based on hybrid[4]arene and 1,2,4,5-tetracyanobenzene that is able to construct vapochromic materials. After the capture of benzene and toluene vapors, activated hybrid[4]arene-based co-crystal forms new structures, accompanied by color changes from brown to yellow. However, when hybrid[4]arene-based co-crystal captures cyclohexane and pyridine, neither structures nor colors change. Interestingly, hybrid[4]arene-based co-crystal can separate benzene from a benzene/cyclohexane equal-volume mixture and allow toluene to be removed from a toluene/ pyridine equal-volume mixture with purities reaching 100%. In addition, the process of adsorptive separation can be visually monitored. The selectivity of benzene from a benzene/cyclohexane equal-volume mixture and toluene from a toluene/ pyridine equal-volume mixture is attributed to the different changes in the charge-transfer interaction between hybrid[4]arene and 1,2,4,5-tetracyanobenzene when hybrid[4]arene-based co-crystal captures different vapors. Moreover, hybrid[4]arene-based co-crystal can be reused without losing selectivity and performance. This work constructs a vapochromic material for hydrocarbon separation.
大环化学与共晶工程的结合推动了超分子科学中具有气致变色行为的材料的发展。在此,我们开发了一种基于杂化[4]芳烃和1,2,4,5-四氰基苯的大环共晶,它能够构建气致变色材料。在捕获苯和甲苯蒸气后,活化的基于杂化[4]芳烃的共晶形成新的结构,同时伴随着颜色从棕色变为黄色。然而,当基于杂化[4]芳烃的共晶捕获环己烷和吡啶时,结构和颜色均未发生变化。有趣的是,基于杂化[4]芳烃的共晶可以从苯/环己烷等体积混合物中分离出苯,并能从甲苯/吡啶等体积混合物中除去甲苯,纯度可达100%。此外,吸附分离过程可以通过视觉进行监测。从苯/环己烷等体积混合物中对苯的选择性以及从甲苯/吡啶等体积混合物中对甲苯的选择性归因于当基于杂化[4]芳烃的共晶捕获不同蒸气时,杂化[4]芳烃与1,2,4,5-四氰基苯之间电荷转移相互作用的不同变化。此外,基于杂化[4]芳烃的共晶可以重复使用而不会丧失选择性和性能。这项工作构建了一种用于烃类分离的气致变色材料。