Gu Xiaoyu, Yan Dong, Zhang Zongxun, Liu Zhengwei, Jing Cheng, Meng Xianyun, Liu Yafei
School of Petroleum Engineering, Xi'an Shiyou University, Xi'an 710065, China.
Engineering Research Center of Development and Management for Low to Extra-Low Permeability Oil & Gas Reservoirs in West China, Ministry of Education, Xi'an, Shaanxi 710065, China.
ACS Omega. 2024 Jan 23;9(5):5705-5714. doi: 10.1021/acsomega.3c07860. eCollection 2024 Feb 6.
The efficiency of reservoir imbibition in continental tight sandstone reservoirs is severely hindered due to their intricate wettability characteristics. To address this challenge, we propose a novel synergistic approach that combines low-frequency vibration and nanofluid treatment. This method integrates physical shear and chemical wettability alteration to effectively modify the wettability of neutral oil-wet tight sandstone, thereby enhancing the imbibition process. In this study, we formulated a TX-100 nanofluid system through physical modification. By utilizing the contact angle as a benchmark for evaluation, we investigated the impact of low-frequency fluctuations on the wettability of oil-wet sandstone. Subsequently, we identified the optimal combination of wave parameters. Through isothermal adsorption experiments and mechanical analyses of oil droplets subjected to fluctuations, we systematically elucidated the mechanism by which fluctuations collaborate with nanofluids to alter the wettability of oil-wet sandstone. Furthermore, we evaluated the oil displacement efficiency of cores subjected to the combined action of low-frequency fluctuations and nanofluid treatment. Our findings revealed that the TX-100 nanofluid reduced the static contact angle of oil-wet sandstone by 58%. When assisted by the optimal fluctuation parameters, the nanofluid treatment contributed to a 64% reduction in the contact angle of strongly oil-wet sandstone. This effect further amplified the reversal of wettability in oil-wet sandstone. Through the application of various wave-assisted treatment agents, the efficiency of oil removal was increased by a minimum of 16%. Moreover, the recovery degree of wave-assisted nanofluid imbibition experienced a remarkable enhancement of 30.39%. Nuclear magnetic resonance analysis demonstrated a significant improvement in pore sizes smaller than 1 μm as a result of the composite process.
由于陆相致密砂岩储层复杂的润湿性特征,其储层渗吸效率受到严重阻碍。为应对这一挑战,我们提出了一种将低频振动与纳米流体处理相结合的新型协同方法。该方法整合了物理剪切和化学润湿性改变,以有效改变中性油湿致密砂岩的润湿性,从而增强渗吸过程。在本研究中,我们通过物理改性配制了TX - 100纳米流体体系。以接触角作为评估基准,研究了低频波动对油湿砂岩润湿性的影响。随后,确定了波参数的最佳组合。通过等温吸附实验和对受波动影响的油滴进行力学分析,系统地阐明了波动与纳米流体协同改变油湿砂岩润湿性的机制。此外,我们评估了经低频波动和纳米流体处理联合作用的岩心的驱油效率。我们的研究结果表明,TX - 100纳米流体使油湿砂岩的静态接触角降低了58%。当辅以最佳波动参数时,纳米流体处理使强油湿砂岩的接触角降低了64%。这种效果进一步放大了油湿砂岩润湿性的反转。通过应用各种波辅助处理剂,除油效率至少提高了16%。此外,波辅助纳米流体渗吸的采收程度显著提高了30.39%。核磁共振分析表明,复合过程使小于1μm的孔径有了显著改善。