Kearney Luke M, Katz Richard F, MacMinn Christopher W, Kirkham Chris, Cartwright Joe
Department of Earth Sciences, University of Oxford, Oxford OX1 3AN, United Kingdom.
Department of Engineering Science, University of Oxford, Oxford OX1 3PJ, United Kingdom.
Proc Natl Acad Sci U S A. 2024 Feb 20;121(8):e2312152121. doi: 10.1073/pnas.2312152121. Epub 2024 Feb 12.
Subsurface sandstone reservoirs sealed by overlying, low-permeability layers provide capacity for long-term sequestration of anthropogenic waste. Leakage can occur if reservoir pressures rise sufficiently to fracture the seal. Such pressures can be generated within the reservoir by vigorous injection of waste or, over thousands of years, by natural processes. In either case, the precise role of intercalated mudstones in the long-term evolution of reservoir pressure remains unclear; these layers have variously been viewed as seals, as pressure sinks, or as pressure sources. Here, we use the geological record of episodic fluid venting in the Levant Basin to provide striking evidence for the pressure-source hypothesis. We use a Bayesian framework to combine recently published venting data, which record critical subsurface pressures since ∼2 Ma, with a stochastic model of pressure evolution to infer a pressure-recharge rate of ∼30 MPa/Myr. To explain this large rate, we quantify and compare a range of candidate mechanisms. We find that poroelastic pressure diffusion from mudstones provides the most plausible explanation for these observations, amplifying the ∼3 MPa/Myr recharge caused primarily by tectonic compression. Since pressurized mudstones are ubiquitous in sedimentary basins, pressure diffusion from mudstones is likely to promote seal failure globally.
被上覆低渗透层封闭的地下砂岩储层具备长期封存人为废弃物的能力。如果储层压力上升到足以使密封层破裂,就可能发生泄漏。通过大量注入废弃物或者历经数千年的自然过程,储层内部会产生这样的压力。无论哪种情况,夹层泥岩在储层压力长期演化过程中的确切作用仍不清楚;这些岩层被分别视作密封层、压力汇或压力源。在此,我们利用黎凡特盆地间歇性流体排放的地质记录,为压力源假说提供了有力证据。我们采用贝叶斯框架,将最近发表的排放数据(记录了自约200万年前以来的关键地下压力)与压力演化的随机模型相结合,推断出压力补给速率约为30兆帕/百万年。为解释这一高补给速率,我们对一系列候选机制进行了量化和比较。我们发现,泥岩的孔隙弹性压力扩散为这些观测结果提供了最合理的解释,放大了主要由构造压缩引起的约3兆帕/百万年的补给量。由于承压泥岩在沉积盆地中普遍存在,泥岩的压力扩散可能在全球范围内促使密封层失效。