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使用氧化石墨烯修饰的聚醚砜膜增强从污染水中去除铁(Fe)和锰(Mn)离子:合成与表征

Enhanced removal of iron (Fe) and manganese (Mn) ions from contaminated water using graphene oxide-decorated polyethersulphone membranes: Synthesis and characterization.

作者信息

Goyat Rohit, Singh Joginder, Umar Ahmad, Ibrahim Ahmed A, Kumari Savita, Malik Sumit, Chaudhary Vivek, Akbar Sheikh, Baskoutas Sotirios

机构信息

Department of Chemistry, Maharishi Markandeshwar (Deemed to be University), Mullana, Ambala, Haryana, India.

Department of Chemistry, College of Science and Arts, and Promising Centre for Sensors and Electronic Devices (PCSED), Najran University, Najran, Kingdom of Saudi Arabia.

出版信息

Waste Manag Res. 2024 Aug;42(8):608-617. doi: 10.1177/0734242X241227379. Epub 2024 Feb 14.

DOI:10.1177/0734242X241227379
PMID:38353237
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11295411/
Abstract

This study addresses the urgent issue of water pollution caused by iron (Fe) and manganese (Mn) ions. It introduces an innovative approach using graphene oxide (GO) and GO-decorated polyethersulphone (PES) membranes to efficiently remove these ions from contaminated water. The process involves integrating GO into PES membranes to enhance their adsorption capacity. Characterization techniques, including scanning electron microscopy, Fourier-transform infrared, and contact angle measurements, were used to assess structural and surface properties. The modified membranes demonstrated significantly improved adsorption compared to pristine PES. Notably, they achieved over 94% removal of Mn and 93.6% of Fe in the first filtration cycle for water with an initial concentration of 100 ppm. Continuous filtration for up to five cycles maintained removal rates above 60%. This research advances water purification materials, offering a promising solution for heavy metal ion removal. GO-decorated PES membranes may find application in large-scale water treatment, addressing environmental and public health concerns.

摘要

本研究解决了由铁(Fe)和锰(Mn)离子引起的水污染这一紧迫问题。它介绍了一种创新方法,即使用氧化石墨烯(GO)和GO修饰的聚醚砜(PES)膜从受污染水中有效去除这些离子。该过程包括将GO整合到PES膜中以提高其吸附能力。使用包括扫描电子显微镜、傅里叶变换红外光谱和接触角测量在内的表征技术来评估结构和表面性质。与原始PES相比,改性膜的吸附性能有显著改善。值得注意的是,对于初始浓度为100 ppm的水,它们在第一个过滤循环中实现了超过94%的Mn去除率和93.6%的Fe去除率。连续过滤多达五个循环,去除率保持在60%以上。这项研究推动了水净化材料的发展,为重金属离子去除提供了一个有前景的解决方案。GO修饰的PES膜可能会在大规模水处理中得到应用,解决环境和公共卫生问题。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d170/11295411/770dcc4df652/10.1177_0734242X241227379-fig5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d170/11295411/65479950e5e5/10.1177_0734242X241227379-fig1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d170/11295411/9ac816531f18/10.1177_0734242X241227379-fig2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d170/11295411/d92ae15d8236/10.1177_0734242X241227379-fig3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d170/11295411/60e40f8e6264/10.1177_0734242X241227379-fig4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d170/11295411/770dcc4df652/10.1177_0734242X241227379-fig5.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d170/11295411/65479950e5e5/10.1177_0734242X241227379-fig1.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d170/11295411/9ac816531f18/10.1177_0734242X241227379-fig2.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d170/11295411/d92ae15d8236/10.1177_0734242X241227379-fig3.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d170/11295411/60e40f8e6264/10.1177_0734242X241227379-fig4.jpg
https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d170/11295411/770dcc4df652/10.1177_0734242X241227379-fig5.jpg

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