Wang Wenxing, Yao Yu, Xin Jiangang, Zhao Xueling, Xie Lili, Zhu Zhigang
School of Energy and Materials, Shanghai Polytechnic University, Shanghai, 201209, People's Republic of China.
School of Health Science and Engineering, University of Shanghai for Science and Technology, Shanghai, 200093, People's Republic of China.
Nanotechnology. 2024 Mar 6;35(21). doi: 10.1088/1361-6528/ad2b4a.
MXene, a class of two-dimensional materials that are emerging as rising stars in the field of materials, are receiving much attention in sensing. TiCTMXene, the most maturely researched MXene, is widely used in energy, biomedical, laser, and microwave shielding applications and has also been expanded to gas sensing and wearable electronics applications. Compared with TiCT, NbCTMXene is more difficult to etch and has higher resistances at room temperature; so, few studies have been reported on their use in the sensing field. Based on the preparation of few-layer NbCTMXene by intercalation, this study thoroughly examined their gas-sensing properties. The successfully prepared few-layer NbCTshowed good selectivity and high sensitivity to triethylamine at room temperature, with response values up to 47.2% for 50 ppm triethylamine and short response/recovery time (22/20 s). This study opens an important path for the design of novel Nb-based MXene sensors for triethylamine gas detection.
MXene是一类二维材料,在材料领域正崭露头角,在传感方面备受关注。TiCT MXene是研究最为成熟的MXene,广泛应用于能源、生物医学、激光和微波屏蔽应用,并且已扩展到气体传感和可穿戴电子应用。与TiCT相比,NbCT MXene更难蚀刻,在室温下具有更高的电阻;因此,关于其在传感领域应用的研究报道较少。基于通过插层制备少层NbCT MXene,本研究全面考察了它们的气敏特性。成功制备的少层NbCT对三乙胺在室温下表现出良好的选择性和高灵敏度,对于50 ppm三乙胺的响应值高达47.2%,且响应/恢复时间短(22/20 s)。本研究为设计用于三乙胺气体检测的新型Nb基MXene传感器开辟了一条重要途径。