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金属 kagome 亚铁磁体中的反常电子。

Anomalous electrons in a metallic kagome ferromagnet.

机构信息

Paul Scherrer Institute, Villigen, Switzerland.

Department of Quantum Matter Physics, University of Geneva, Geneva, Switzerland.

出版信息

Nature. 2024 Mar;627(8002):67-72. doi: 10.1038/s41586-024-07085-w. Epub 2024 Mar 6.

Abstract

Ordinary metals contain electron liquids within well-defined 'Fermi' surfaces at which the electrons behave as if they were non-interacting. In the absence of transitions to entirely new phases such as insulators or superconductors, interactions between electrons induce scattering that is quadratic in the deviation of the binding energy from the Fermi level. A long-standing puzzle is that certain materials do not fit this 'Fermi liquid' description. A common feature is strong interactions between electrons relative to their kinetic energies. One route to this regime is special lattices to reduce the electron kinetic energies. Twisted bilayer graphene is an example, and trihexagonal tiling lattices (triangular 'kagome'), with all corner sites removed on a 2 × 2 superlattice, can also host narrow electron bands for which interaction effects would be enhanced. Here we describe spectroscopy revealing non-Fermi-liquid behaviour for the ferromagnetic kagome metal FeSn (ref. ). We discover three C-symmetric electron pockets at the Brillouin zone centre, two of which are expected from density functional theory. The third and most sharply defined band emerges at low temperatures and binding energies by means of fractionalization of one of the other two, most likely on the account of enhanced electron-electron interactions owing to a flat band predicted to lie just above the Fermi level. Our discovery opens the topic of how such many-body physics involving flat bands could differ depending on whether they arise from lattice geometry or from strongly localized atomic orbitals.

摘要

普通金属在定义明确的“费米”表面内包含电子液体,在该表面内,电子的行为似乎是非相互作用的。在没有向完全新的相(如绝缘体或超导体)转变的情况下,电子之间的相互作用会导致散射,这种散射与结合能偏离费米能级的二次方成正比。一个长期存在的难题是,某些材料不符合这种“费米液体”描述。一个常见的特征是电子之间的相互作用相对于它们的动能很强。达到这一状态的一种途径是采用特殊晶格来降低电子动能。扭曲双层石墨烯就是一个例子,而三六边形平铺晶格(三角形“kagome”),在 2×2 的超晶格上移除所有角点,也可以容纳窄带电子,其中相互作用效应会增强。在这里,我们描述了光谱学揭示的铁锡(FeSn)亚铁 kagome 金属的非费米液体行为。我们在布里渊区中心发现了三个 C 对称的电子口袋,其中两个是根据密度泛函理论预测的。第三个也是最清晰的能带在低温和结合能下出现,是通过另两个能带的分数化产生的,最有可能是由于预测存在于费米能级上方的平带导致的电子-电子相互作用增强。我们的发现开辟了一个主题,即涉及平带的这种多体物理如何因它们是由晶格几何还是由强局域原子轨道引起而有所不同。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/546d/10917658/fa337f9d43e6/41586_2024_7085_Fig1_HTML.jpg

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