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用于预测印度贾杜达铀矿尾矿中氡通量的数值模型。

A numerical model for the prediction of radon flux from uranium mill tailings at Jaduguda, India.

机构信息

Health Physics Unit, Bhabha Atomic Research Centre, Jaduguda, 832102, Jharkhand, India.

Health Physics Division, Bhabha Atomic Research Centre, Trombay, 400094, Maharastra, India.

出版信息

Environ Sci Pollut Res Int. 2024 Apr;31(17):24951-24960. doi: 10.1007/s11356-024-32674-7. Epub 2024 Mar 9.

Abstract

Solid process fine waste or tailings of a uranium mill is a potential source of release of radiologically significant gaseous radon (Rn). A number of variables such as radium (Ra) content, porosity, moisture content, and tailings density can affect the extent of emanation from the tailings. Further, if a cover material is used for remediation purposes, additional challenges due to changes in the matrix characteristics in predicting the radon flux can be anticipated. The uranium mill tailings impoundment systems at Jaduguda have been in use for the long-term storage of fine process waste (tailings). A pilot-scale remediation exercise of one of the tailings ponds has been undertaken with 30 cm soil as a cover material. For the prediction of the radon flux, a numerical model has been developed to account for the radon exhalation process at the remediated site. The model can effectively be used to accommodate both the continuous and discrete variable inputs. Depth profiling and physicochemical characterization for the remediated site have been done for the required input variables of the proposed numerical model. The predicted flux worked out is well below the reference level of 0.74 Bq m s IAEA (2004).

摘要

铀矿加工厂的固体工艺废料或尾矿是放射性气体氡(Rn)释放的潜在来源。镭(Ra)含量、孔隙率、含水量和尾矿密度等多个变量会影响尾矿的散发程度。此外,如果使用覆盖材料进行修复,由于预测氡通量时基质特性的变化,可能会带来额外的挑战。贾杜古达铀矿加工厂的尾矿库系统长期用于储存精细工艺废料(尾矿)。对其中一个尾矿池进行了试点规模的修复,使用 30 厘米厚的土壤作为覆盖材料。为了预测氡通量,开发了一个数值模型来考虑修复现场的氡排放过程。该模型可以有效地适应连续和离散变量的输入。已对修复现场进行了深度剖析和物理化学特性分析,以获取所提议的数值模型的所需输入变量。计算得出的预测通量远低于 0.74 Bq m s IAEA(2004 年)的参考水平。

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