State Key Laboratory of Bioactive Substance and Function of Natural Medicines, Institute of Materia Medica, Chinese Academy of Medical Sciences and Peking Union Medical College, Xian Nong Tan Street, Beijing, 100050, P. R. China.
Key Laboratory of Preclinical Study for New Drugs of Gansu Province, School of Basic Medical Sciences and Research Unit of Peptide Science, Chinese Academy of Medical Sciences, Lanzhou University, 199 West Donggang Road, Lanzhou, Gansu, 730000, P. R. China.
Adv Sci (Weinh). 2024 Jun;11(21):e2308491. doi: 10.1002/advs.202308491. Epub 2024 Mar 11.
Peptide and protein postmodification have gained significant attention due to their extensive impact on biomolecule engineering and drug discovery, of which cysteine-specific modification strategies are prominent due to their inherent nucleophilicity and low abundance. Herein, the study introduces a novel approach utilizing multifunctional 5-substituted 1,2,3-triazine derivatives to achieve multifaceted bioconjugation targeting cysteine-containing peptides and proteins. On the one hand, this represents an inaugural instance of employing 1,2,3-triazine in biomolecular-specific modification within a physiological solution. On the other hand, as a powerful combination of precision modification and biorthogonality, this strategy allows for the one-pot dual-orthogonal functionalization of biomolecules utilizing the aldehyde group generated simultaneously. 1,2,3-Triazine derivatives with diverse functional groups allow conjugation to peptides or proteins, while bi-triazines enable peptide cyclization and dimerization. The examination of the stability of bi-triazines revealed their potential for reversible peptide modification. This work establishes a comprehensive platform for identifying cysteine-selective modifications, providing new avenues for peptide-based drug development, protein bioconjugation, and chemical biology research.
由于肽和蛋白质的翻译后修饰对生物分子工程和药物发现有广泛的影响,因此引起了人们的极大关注,其中半胱氨酸特异性修饰策略因其固有的亲核性和低丰度而引人注目。本文介绍了一种利用多功能 5-取代 1,2,3-三嗪衍生物实现针对含半胱氨酸肽和蛋白质的多方位生物偶联的新方法。一方面,这代表了在生理溶液中首次将 1,2,3-三嗪用于生物分子特异性修饰。另一方面,作为精确修饰和生物正交性的强大组合,该策略允许利用同时生成的醛基一锅法对生物分子进行双正交功能化。具有各种官能团的 1,2,3-三嗪衍生物可与肽或蛋白质进行缀合,而双三嗪可使肽环化和二聚化。对双三嗪稳定性的研究表明,它们可用于可逆肽修饰。这项工作为鉴定半胱氨酸选择性修饰建立了一个全面的平台,为基于肽的药物开发、蛋白质生物偶联和化学生物学研究提供了新途径。