Kokalj Jure
Department of Theoretical Physics, Jožef Stefan Institute, Ljubljana 1000, Slovenia.
Faculty of Civil and Geodetic Engineering, Department of Mathematics and Physics, University of Ljubljana, Ljubljana 1000, Slovenia.
Proc Natl Acad Sci U S A. 2024 Mar 19;121(12):e2322670121. doi: 10.1073/pnas.2322670121. Epub 2024 Mar 12.
The bad metallic phase with resistivity above the Mott-Ioffe-Regel (MIR) limit, which appears also in cuprate superconductors, was recently understood by cold atom and computer simulations of the Hubbard model via charge susceptibility and charge diffusion constant. However, since reliable simulations can be typically done only at temperatures above the experimental temperatures, the question for cuprate superconductors is still open. This paper addresses this question by resorting to heat transport, which allows for the estimate of electronic diffusion and it further combines it with the resistivity to estimate the charge susceptibility. The doping and temperature dependencies of diffusion constant and charge susceptibilities are shown and discussed for two samples of YBaCuO. Results indicate strongly incoherent transport, mean free path corresponding to the MIR limit for the underdoped sample at temperatures above ~200 K and significant effect of the charge susceptibility on the resistivity.
电阻率高于莫特-约菲-雷格尔(MIR)极限的不良金属相,同样出现在铜酸盐超导体中,最近通过哈伯德模型的冷原子和计算机模拟,借助电荷磁化率和电荷扩散常数得以理解。然而,由于可靠的模拟通常只能在高于实验温度的温度下进行,铜酸盐超导体的问题仍然悬而未决。本文通过采用热传输来解决这个问题,热传输能够对电子扩散进行估计,并进一步将其与电阻率相结合以估计电荷磁化率。针对钇钡铜氧(YBaCuO)的两个样品,展示并讨论了扩散常数和电荷磁化率的掺杂及温度依赖性。结果表明存在强烈的非相干输运,对于欠掺杂样品,在温度高于约200 K时,平均自由程对应于MIR极限,并且电荷磁化率对电阻率有显著影响。