Simon C, Silevitch D M, Stamp P C E, Rosenbaum T F
Division of Physics, Mathematics, and Astronomy, California Institute of Technology, Pasadena, CA 91125.
Department of Physics and Astronomy, University of British Columbia, Vancouver, BC V6T 1Z1, Canada.
Proc Natl Acad Sci U S A. 2024 Mar 26;121(13):e2315598121. doi: 10.1073/pnas.2315598121. Epub 2024 Mar 19.
Most macroscopic magnetic phenomena (including magnetic hysteresis) are typically understood classically. Here, we examine the dynamics of a uniaxial rare-earth ferromagnet deep within the quantum regime, so that domain wall motion, and the associated hysteresis, is initiated by quantum nucleation, which then grows into large-scale domain wall motion, which is observable as an unusual form of Barkhausen noise. We observe noncritical behavior in the resulting avalanche dynamics that only can be explained by going beyond traditional renormalization group methods or classical domain wall models. We find that this "quantum Barkhausen noise" exhibits two distinct mechanisms for domain wall movement, each of which is quantum-mechanical, but with very different dependences on an external magnetic field applied transverse to the spin (Ising) axis. These observations can be understood in terms of the correlated motion of pairs of domain walls, nucleated by cotunneling of plaquettes (sections of domain wall), with plaquette pairs correlated by dipolar interactions; this correlation is suppressed by the transverse field. Similar macroscopic correlations may be expected to appear in the hysteresis of other systems with long-range interactions.
大多数宏观磁现象(包括磁滞)通常用经典理论来理解。在此,我们研究处于量子 regime 深处的单轴稀土铁磁体的动力学,使得畴壁运动以及相关的磁滞由量子成核引发,然后发展为大规模的畴壁运动,这可作为一种不寻常形式的巴克豪森噪声被观测到。我们在由此产生的雪崩动力学中观察到非临界行为,这种行为只能通过超越传统重整化群方法或经典畴壁模型来解释。我们发现这种“量子巴克豪森噪声”展现出两种不同的畴壁运动机制,每一种都是量子力学的,但对垂直于自旋(伊辛)轴施加的外部磁场具有非常不同的依赖性。这些观测结果可以通过畴壁对的关联运动来理解,畴壁对由面元(畴壁的部分)的共隧穿成核,面元对通过偶极相互作用相关联;这种关联被横向场抑制。类似的宏观关联可能会出现在其他具有长程相互作用的系统的磁滞现象中。