Brooke J, Rosenbaum T F, Aeppli G
The James Franck Institute and Department of Physics, The University of Chicago, Chicago, Illinois 60637, USA.
Nature. 2001 Oct 11;413(6856):610-3. doi: 10.1038/35098037.
Perhaps the most anticipated, yet experimentally elusive, macroscopic quantum phenomenon is spin tunnelling in a ferromagnet, which may be formulated in terms of domain wall tunnelling. One approach to identifying such a process is to focus on mesoscopic systems where the number of domain walls is finite and the motion of a single wall has measurable consequences. Research of this type includes magnetotransport measurements on thin ferromagnetic wires, and magnetization experiments on single particles, nanomagnet ensembles and rare-earth multilayers. A second method is to investigate macroscopic disordered ferromagnets, whose dynamics are dominated by domain wall motion, and search the associated relaxation-time distribution functions for the signature of quantum effects. But whereas the classical, thermal processes that operate in these experiments are easily regulated via temperature, the quantum processes have so far not been tunable, making difficult a definitive interpretation of the results in terms of tunnelling. Here we describe a disordered magnetic system for which it is possible to adjust the quantum tunnelling probabilities. For this material, we can model both the classical, thermally activated response at high temperatures and the athermal, tunnelling behaviour at low temperatures within a unified framework, where the domain wall is described as a particle with a fixed mass. We show that it is possible to tune the quantum tunnelling processes by adjusting the 'mass' of this particle with an external magnetic field.
也许最令人期待却在实验中难以捉摸的宏观量子现象是铁磁体中的自旋隧穿,它可以用畴壁隧穿来表述。识别这种过程的一种方法是关注介观系统,其中畴壁的数量是有限的,单个畴壁的运动会产生可测量的结果。这类研究包括对细铁磁线的磁输运测量,以及对单个粒子、纳米磁体集合体和稀土多层膜的磁化实验。第二种方法是研究宏观无序铁磁体,其动力学由畴壁运动主导,并在相关的弛豫时间分布函数中寻找量子效应的特征。但是,尽管在这些实验中起作用的经典热过程可以通过温度轻松调节,但量子过程迄今为止还无法调节,这使得难以根据隧穿对结果进行明确的解释。在这里,我们描述了一种无序磁系统,对于该系统可以调节量子隧穿概率。对于这种材料,我们可以在一个统一的框架内对高温下的经典热激活响应和低温下的无热隧穿行为进行建模,其中畴壁被描述为具有固定质量的粒子。我们表明,可以通过用外部磁场调节该粒子的“质量”来调整量子隧穿过程。