García-Puente Yalina, Auguié Baptiste, Kashyap Raman
Opt Express. 2024 Mar 11;32(6):9644-9655. doi: 10.1364/OE.514259.
This work proposes what we believe to be a novel Tamm plasmon-like resonance supporting structure consisting of an Au/SiO core-shell metal nanosphere structure surrounded by a TiO/SiO spherical Bragg resonator (SBR). The cavity formed between the core metal particle and the SBR supports a localized mode similar to Tamm plasmons in planar dielectric multilayers. Theoretical simulations reveal a sharp absorption peak in the SBR bandgap region, associated with this mode, together with strong local field enhancement. We studied the modification of a dipolar electric emitter's radiative and non-radiative decay rates in this resonant structure, resulting in a quantum efficiency of ∼90% for a dipole at a distance of =60 from the Au nanosphere surface. A 30-layer metal-SBR Tamm plasmon-like resonant supporting structure results in a Q up to ∼10. The Tamm plasmon-like mode is affected by the Bragg wavelength and the number of layers of the SBR, and the thickness of the spacer cavity layer. These results will open a new avenue for generating high-Q Tamm plasmon-like modes for switches, optical logic computing devices, and nonlinear applications.
这项工作提出了一种我们认为新颖的类塔姆等离子体共振支撑结构,它由一个被TiO/SiO球形布拉格谐振器(SBR)包围的Au/SiO核壳金属纳米球结构组成。在核心金属颗粒和SBR之间形成的腔支持一种类似于平面介质多层膜中塔姆等离子体的局域模式。理论模拟揭示了在SBR带隙区域存在一个与该模式相关的尖锐吸收峰,以及强烈的局部场增强。我们研究了在这种共振结构中偶极电发射器的辐射和非辐射衰减率的变化,对于距离金纳米球表面60的偶极,量子效率达到了约90%。一个30层的金属-SBR类塔姆等离子体共振支撑结构的品质因数高达约10。类塔姆等离子体模式受布拉格波长、SBR的层数以及间隔腔层厚度的影响。这些结果将为开关、光学逻辑计算设备和非线性应用产生高Q值类塔姆等离子体模式开辟一条新途径。