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南亚和东南亚控制着青藏高原东南部梅里雪山的黑碳特征。

South and Southeast Asia controls black carbon characteristics of Meili Snow Mountains in southeast Tibetan Plateau.

作者信息

Chen Pengfei, Kang Shichang, Hu Yuling, Pu Tao, Liu Yajun, Wang Shijin, Rai Mukesh, Wang Ke, Tripathee Lekhendra, Li Chaoliu

机构信息

State Key Laboratory of Cryospheric Science, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000, China; University of Chinese Academy of Sciences, Beijing 100049, China.

State Key Laboratory of Cryospheric Science, Northwest Institute of Eco-Environment and Resources, Chinese Academy of Sciences, Lanzhou 730000, China; University of Chinese Academy of Sciences, Beijing 100049, China.

出版信息

Sci Total Environ. 2024 Jun 1;927:172262. doi: 10.1016/j.scitotenv.2024.172262. Epub 2024 Apr 5.

Abstract

South and Southeast Asia (SSA) emitted black carbon (BC) exerts potential effects on glacier and snow melting and regional climate change in the Tibetan Plateau. In this study, online BC measurements were conducted for 1 year at a remote village located at the terminus of the Mingyong Glacier below the Meili Snow Mountains. The Weather Research and Forecasting model coupled with Chemistry (WRF-Chem) was used to investigate the contribution and potential effect of SSA-emitted BC. In addition, variations in the light absorption characteristics of BC and brown carbon (BrC) were examined. The results indicated that the annual mean concentration of BC was 415 ± 372 ngm, with the highest concentration observed in April (monthly mean: 930 ± 484 ngm). BC exhibited a similar diurnal variation throughout the year, with two peaks observed in the morning (from 8:00 to 9:00 AM) and in the afternoon (from 4:00 to 5:00 PM), with even lower values at nighttime. At a short wavelength of 370 nm, the absorption coefficient (b) reached its maximum value, and the majority of b values were < 20 Mm, indicating that the atmosphere was not overloaded with BC. At the same wavelength, BrC substantially contributed to b, with an annual mean of 25.2 % ± 12.8 %. SSA was the largest contributor of BC (annual mean: 51.1 %) in the study area, particularly in spring (65.6 %). However, its contributions reached 20.2 % in summer, indicating non-negligible emissions from activities in other regions. In the atmosphere, the SSA BC-induced radiative forcing (RF) over the study region was positive. While at the near surface, the RF exhibited a significant seasonal variation, with the larger RF values occurring in winter and spring. Overall, our findings highlight the importance of controlling BC emissions from SSA to protect the Tibetan Plateau against pollution-related glacier and snow cover melting.

摘要

南亚和东南亚排放的黑碳对青藏高原的冰川和积雪融化以及区域气候变化具有潜在影响。在本研究中,在位于梅里雪山明永冰川末端的一个偏远村庄进行了为期一年的黑碳在线测量。利用耦合化学的气象研究与预报模型(WRF-Chem)来研究南亚和东南亚排放的黑碳的贡献及潜在影响。此外,还研究了黑碳和棕碳(BrC)光吸收特性的变化。结果表明,黑碳的年平均浓度为415±372 ng/m³,4月观测到的浓度最高(月平均:930±484 ng/m³)。黑碳全年呈现相似的日变化,在上午(8:00至9:00)和下午(4:00至5:00)出现两个峰值,夜间值更低。在370 nm的短波长下,吸收系数(b)达到最大值,且大多数b值<20 Mm,表明大气中黑碳未过载。在同一波长下,棕碳对b有显著贡献,年平均值为25.2%±12.8%。南亚和东南亚是研究区域黑碳的最大贡献源(年平均:51.1%),特别是在春季(65.6%)。然而,其在夏季的贡献达到20.2%,表明其他地区活动的排放也不可忽视。在大气中,南亚和东南亚黑碳引起的研究区域辐射强迫(RF)为正值。而在近地表,辐射强迫呈现显著的季节变化,冬季和春季的辐射强迫值较大。总体而言,我们的研究结果凸显了控制南亚和东南亚黑碳排放对于保护青藏高原免受与污染相关的冰川和积雪融化影响的重要性。

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