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使用便携式平面高纯锗探测器估算组织中嵌入的 241Am 和 239Pu 活度。

Estimation of 241Am and 239Pu activity embedded in the tissue using portable planar HPGe detector.

机构信息

Safety, Quality and Resource Management Group, Indira Gandhi Centre for Atomic Research, Kalpakkam 603012, Tamilnadu, India.

出版信息

Radiat Prot Dosimetry. 2024 Jun 3;200(8):721-738. doi: 10.1093/rpd/ncae105.

Abstract

This paper describes a procedure for the estimation of 241Am and 239Pu activity present in the human tissue by measuring the depth of contaminant using a portable Planar High Purity Germanium detector (HPGe). The ratios of photopeak counts of X-rays or gammas obtained with the detector coupled to collimator are calculated for the estimation of depth of the contaminant and the optimum one is determined. Since Minimum Detectable Activities (MDA) for the detector coupled to a collimator are higher than that of bare detector, activity must be estimated using bare detector, after locating the contaminant. Two methods are described for the estimation of plutonium coexisting with 241Am: (i) Abundance and isotopic correction for 239Pu (ii) and 239Pu:241Am ratio. The procedure to estimate 239Pu when plutonium isotopes alone are present is also established. An optimum monitoring period to detect the minimum value of intake for both radionuclides corresponding to chelation therapy and excision is also derived.

摘要

本文描述了一种使用便携式平面高纯锗探测器 (HPGe) 通过测量污染物深度来估算人体组织中 241Am 和 239Pu 活度的方法。对于估算污染物深度,计算了与准直器耦合的探测器获得的 X 射线或伽马射线光电峰计数比,并确定了最佳比。由于与准直器耦合的探测器的最小可探测活度 (MDA) 高于裸探测器,因此必须在定位污染物后使用裸探测器估计活度。描述了两种估算与 241Am 共存的钚的方法:(i) 239Pu 的丰度和同位素校正 (ii) 和 239Pu:241Am 比。还建立了仅存在钚同位素时估算 239Pu 的程序。还推导出了检测螯合疗法和切除对应于两种放射性核素的摄入最小值的最佳监测期。

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