Department of Meteorology and Geophysics, University of Vienna, Universitätsring 1, Vienna 1010, Austria.
Environ Sci Technol. 2024 Jun 4;58(22):9741-9749. doi: 10.1021/acs.est.4c01252. Epub 2024 May 20.
Microplastics (MPs) are emerging as an atmospheric pollutant. Here, we present a method of estimating MP resuspension with mineral dust in bare soil based on reported MP mass in soils, their enrichment in suspended dust relative to soil, and a mineral dust resuspension scheme. Using the estimated resuspensions, we simulate the global atmospheric MP transport and deposition using the dispersion model FLEXPART for two particle shape scenarios, spheres, and fibers. We estimate the uncertainties using a Monte Carlo technique that varies input data parameters within their reported ranges. The total MP resuspensions are estimated at about 104 (48-110) tonnes yr. We find that bare soils in West Asia and North Africa are the main source regions. FLEXPART results show that fibers have higher concentrations in the atmosphere and are dispersed more widely than spheres. Annually, 75 (43-83) tonnes of microfibers are deposited on land and 29 (18-33) tonnes in the oceans. Resuspended MPs can even reach remote regions, such as the Arctic. The results suggest that areas with bare soils can be an important MP source; however, further research on the factors that affect resuspension is needed.
微塑料(MPs)正在成为一种大气污染物。在这里,我们提出了一种基于土壤中报道的 MPs 质量、它们在悬浮尘中相对于土壤的富集程度以及矿物尘埃再悬浮方案来估算裸土中 MPs 与矿物尘埃再悬浮的方法。使用估算的再悬浮量,我们使用扩散模型 FLEXPART 模拟了全球大气 MPs 的传输和沉积,采用了两种颗粒形状情景,即球体和纤维。我们使用蒙特卡罗技术来估计不确定性,该技术在报告的范围内变化输入数据参数。总的 MPs 再悬浮量估计约为 104(48-110)吨/年。我们发现西亚和北非的裸土是主要的源区。FLEXPART 的结果表明,纤维在大气中的浓度更高,比球体分布更广。每年,75(43-83)吨微纤维沉积在陆地上,29(18-33)吨沉积在海洋中。再悬浮的 MPs 甚至可以到达北极等偏远地区。结果表明,裸土地区可能是 MPs 的一个重要来源;然而,需要进一步研究影响再悬浮的因素。