Fermi Andrea, D'Agostino Simone, Dai Yasi, Brunetti Filippo, Negri Fabrizia, Gingras Marc, Ceroni Paola
Dipartimento di Chimica "Giacomo Ciamician", Alma Mater Studiorum -, Università di Bologna, Via Selmi 2, 40126, Bologna, Italy.
Aix-Marseille Université, CNRS, CINaM, 163 Av. de Luminy, 13009 -, Marseille, France.
Chemistry. 2024 Aug 1;30(43):e202401768. doi: 10.1002/chem.202401768. Epub 2024 Jul 11.
Room temperature phosphorescence rarely occurs from pure organic molecules, especially in the solid-state. A strategy for the design of highly emissive organic phosphors is still hard to predict, thus impeding the development of new functional materials with the desired optical properties. Herein, we analyze a family of alkyl and aryl-substituted persulfurated benzenes, the latter representing a class of organic solid-state triplet emitters able to show very high emission quantum yield at room temperature. In this work, we correlate structural parameters with the photophysical properties observed in different experimental conditions (diluted solution, crystalline and amorphous phase at RT and low temperature). Our results, corroborated by a detailed computational analysis, indicate a close relationship between the luminescence properties and i) the nature of the substituents on the persulfurated core, ii) the adopted conformations in the solid state, both in crystalline and amorphous phases. These factors contribute to characterize the lowest-energy lying excited-state, its deactivation pathways, the phosphorescence lifetime and quantum yield. These findings provide a useful roadmap for the development of highly performing purely organic solid-state emitters based on the persulfurated benzene platform.
室温磷光很少发生于纯有机分子,尤其是在固态中。设计高发射有机磷光体的策略仍然难以预测,从而阻碍了具有所需光学性质的新型功能材料的开发。在此,我们分析了一系列烷基和芳基取代的过硫化苯,后者代表一类有机固态三重态发射体,能够在室温下表现出非常高的发射量子产率。在这项工作中,我们将结构参数与在不同实验条件(稀释溶液、室温及低温下的晶相和非晶相)下观察到的光物理性质相关联。我们的结果得到详细计算分析的证实,表明发光性质与以下因素密切相关:i)过硫化核心上取代基的性质;ii)在固态中,无论是晶相还是非晶相中所采用的构象。这些因素有助于表征最低能量的激发态、其失活途径、磷光寿命和量子产率。这些发现为基于过硫化苯平台开发高性能纯有机固态发射体提供了有用的路线图。