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使用耗散粒子动力学研究阴离子和非离子表面活性剂复配微乳液的表面活性剂协同效应及界面性质

Surfactant Synergistic Effect and Interfacial Properties of Microemulsions Compounded with Anionic and Nonionic Surfactants Using Dissipative Particle Dynamics.

作者信息

Zhang Biao, Guan Baoshan, Tao Yufan, Liu Weidong, Peng Baoliang, Lv Kai

机构信息

Research Institute of Percolation Fluids Mechanics, Chinese Academy of Sciences, Beijing 100010, China.

Research Institute of Petroleum Exploration and Development, Beijing 100010, China.

出版信息

ACS Omega. 2024 May 21;9(22):23903-23916. doi: 10.1021/acsomega.4c01933. eCollection 2024 Jun 4.

DOI:10.1021/acsomega.4c01933
PMID:38854575
原文链接:https://pmc.ncbi.nlm.nih.gov/articles/PMC11154924/
Abstract

Microemulsions are one of the most promising directions in enhanced oil recovery, but conventional screening methods are time-consuming and labor-intensive and lack the means to analyze them at the microscopic level. In this paper, we used the Clint model to predict the changes in the synergistic effect of the mixed system of anionic surfactant sodium dodecyl benzenesulfonate and nonionic surfactant polyethoxylated fatty alcohols (C12E6), generated microemulsions using surfactant systems with different mole fractions, and used particle size to analyze the performance and stability of microemulsions, analyze the properties and stability of microemulsions using particle size, and analyze the interfacial behaviors and changes of microemulsions when different systems constitute microemulsions from the point of view of mesoscopic microemulsion self-assembly behaviors by combining with dissipative particle dynamics. It has been shown that microemulsion systems generated from anionic and nonanionic surfactants with a synergistic effect, based on the Clint model, exhibit excellent performance and stability at the microscopic level. The method proposed in this paper can dramatically improve the screening efficiency of microemulsions of anionic and nonanionic surfactants and accurately analyze the properties of microemulsions, so as to provide a theoretical basis for the subsequent research on microemulsions.

摘要

微乳液是提高采收率最有前景的方向之一，但传统的筛选方法耗时费力，且缺乏在微观层面分析它们的手段。在本文中，我们使用克林特模型预测阴离子表面活性剂十二烷基苯磺酸钠和非离子表面活性剂聚乙氧基化脂肪醇（C12E6）混合体系协同效应的变化，使用不同摩尔分数的表面活性剂体系制备微乳液，并利用粒径分析微乳液的性能和稳定性，结合耗散粒子动力学从介观微乳液自组装行为的角度分析微乳液的性质和稳定性以及不同体系形成微乳液时微乳液的界面行为和变化。结果表明，基于克林特模型，由具有协同效应的阴离子和非离子表面活性剂生成的微乳液体系在微观层面表现出优异的性能和稳定性。本文提出的方法可以显著提高阴离子和非离子表面活性剂微乳液的筛选效率，并准确分析微乳液的性质，从而为后续微乳液的研究提供理论依据。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8dee/11154924/3602cf36437f/ao4c01933_0011.jpg
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https://cdn.ncbi.nlm.nih.gov/pmc/blobs/8dee/11154924/16e0d1ef6c86/ao4c01933_0007.jpg
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Monitoring the formation kinetics of a bicontinuous microemulsion.
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