Ng Ryan C, El Sachat Alexandros, Jaramillo-Fernandez Julianna, Sotomayor-Torres Clivia M, Chavez-Angel Emigdio
Catalan Institute of Nanoscience and Nanotechnology (ICN2), CSIC and BIST, Campus UAB, 08193 Bellaterra, Barcelona, Spain.
Institute of Nanoscience and Nanotechnology, National Center for Scientific Research "Demokritos", Agia Paraskevi, 15341 Athens, Greece.
ACS Appl Opt Mater. 2023 Sep 29;2(6):973-979. doi: 10.1021/acsaom.3c00235. eCollection 2024 Jun 28.
This experimental study investigates thermal rectification via asymmetric far-field thermal radiation on a fused silica slab. An asymmetrical distribution of surface emissivity is created over the device by partially covering the fused silica with a 100 nm thick aluminum film. The slab is subjected to a thermal bias, and when this bias is reversed, a small temperature difference is observed between the different configurations. This temperature difference arises from the difference in emissivity between the aluminum layer and fused silica, resulting in the transfer of thermal energy to the surrounding environment through radiation. Experimental findings are supported by finite element simulations, which not only confirm the measured values but also provide valuable insights into the rectification efficiency of the system. The rectification efficiency is found to be approximately 50% at room temperature for a thermal bias of 140 K. Simulations, which are performed by considering different environmental conditions experienced by the radiation and free convection processes, provide further insight into the underlying thermal rectification mechanism. These simulations consider an environmental temperature of 4 K for thermal radiation and an ambient temperature of 294 K for free convection and reveal an enhanced rectification effect with a rectification efficiency up to 600% when a thermal bias of 195 K is applied. This result emphasizes the significance of considering both convection and radiation in the thermal management and rectification of asymmetric systems. The outcomes of this study further our understanding of the thermal rectification phenomenon. They also show the importance of system asymmetry, emissivity disparities, environmental conditions, and the interplay between convection and radiation. Furthermore, the findings have implications for heat transfer and rectification in asymmetric systems, offering potential applications in areas such as energy harvesting, thermal management, and heat transfer optimization in electronic devices.
本实验研究通过在熔融石英平板上进行非对称远场热辐射来研究热整流。通过用100纳米厚的铝膜部分覆盖熔融石英,在器件上形成表面发射率的非对称分布。平板受到热偏置,当该偏置反向时,在不同配置之间观察到小的温差。这种温差源于铝层和熔融石英之间发射率的差异,导致热能通过辐射传递到周围环境。有限元模拟支持了实验结果,该模拟不仅证实了测量值,还为系统的整流效率提供了有价值的见解。对于140 K的热偏置,室温下的整流效率约为50%。通过考虑辐射和自由对流过程所经历的不同环境条件进行的模拟,进一步深入了解了潜在的热整流机制。这些模拟考虑了热辐射的环境温度为4 K,自由对流的环境温度为294 K,并揭示了在施加195 K的热偏置时,整流效率高达600%的增强整流效果。这一结果强调了在非对称系统的热管理和整流中同时考虑对流和辐射的重要性。本研究的结果进一步加深了我们对热整流现象的理解。它们还表明了系统不对称性、发射率差异、环境条件以及对流与辐射之间相互作用的重要性。此外,这些发现对非对称系统中的传热和整流具有启示意义,在能量收集、热管理以及电子设备中的传热优化等领域具有潜在应用。