Pour Haddadan Fahimeh Karimi
Faculty of Physics, Kharazmi University, Tehran 15815-3587, Iran.
J Phys Condens Matter. 2024 Aug 12;36(45). doi: 10.1088/1361-648X/ad69f1.
We consider an active nematic phase and use hydrodynamical equations of it to model the activity as an internal field. The interaction of this field with the nematic director in a confined geometry is included in the Hamiltonian of the system. Based on this model Hamiltonian and the standard field theoretical approach, the Casimir-like force induced between the boundaries of such a confined film is discussed. The force depends on the geometrical shape and the dynamical character of the constituents of our active phase, as well as the anchoring conditions. For homeotropically aligned rod-like particles which in principle tend to align along a planar flow field, extensile activity enhances the attraction present in a thin nematic film. As the film thickness increases the force reduces. Beyond a critical thickness, a planar flow field instantaneous to a bend distortion sets in. Near but below the threshold of this activity-induced instability, the force crosses zero and repulsively diverges right at the critical threshold of this so-called flow instability. For contractile rods, in the same geometry as above, the structure is stable and the Casimir-like force diminishes by an exponential factor as a function of the film thickness. On the other side for a planar director alignment, rod-like contractile particles can induce opposite shear flows at the boundaries creating a splay distortion for the director between the plates. In this configuration, we obtain the same universal pretransitional behavior for the force as above. Vice versa, for extensile rod-like particles in this geometry, the director fluctuations become massive and the Casimir-like force diminishes again by an exponential factor as the film thickness increases. The effect of the active field on thermal fluctuations of the director and the fluctuation-induced Casimir force per area is derived through a "semi"-dynamical approach as well. However, the results of the calculation due to a mathematical sum over the fluctuating modes do not lead to an approved closed form.
我们考虑一种活性向列相,并使用其流体动力学方程将活性建模为一个内场。该场与受限几何结构中向列指向矢的相互作用包含在系统的哈密顿量中。基于此模型哈密顿量和标准场论方法,讨论了这种受限薄膜边界之间诱导的类卡西米尔力。该力取决于活性相成分的几何形状和动力学特性,以及锚定条件。对于垂直排列的棒状粒子,原则上它们倾向于沿平面流场排列,拉伸活性增强了薄向列薄膜中存在的吸引力。随着薄膜厚度增加,力减小。超过临界厚度时,会出现一个瞬间转变为弯曲畸变的平面流场。在这个由活性诱导的不稳定性阈值附近但低于该阈值时,力在这个所谓的流动不稳定性的临界阈值处穿过零并排斥性发散。对于收缩棒,在与上述相同的几何结构中,结构是稳定的,类卡西米尔力随薄膜厚度呈指数因子减小。另一方面,对于平面指向矢排列,棒状收缩粒子可在边界处诱导相反的剪切流,在平板之间的指向矢中产生展曲畸变。在这种构型中,我们得到了与上述相同的力的通用预转变行为。反之,对于这种几何结构中的拉伸棒状粒子,指向矢涨落变得显著,并且随着薄膜厚度增加,类卡西米尔力再次呈指数因子减小。活性场对指向矢热涨落和每单位面积涨落诱导的卡西米尔力的影响也通过一种“半”动力学方法推导得出。然而,由于对涨落模式进行数学求和的计算结果并未得到一个公认的封闭形式。