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铀同位素中子诱发裂变和光致裂变的总激发能分布

Total excitation energy distribution for neutron-induced fission and photo-fission of uranium isotopes.

作者信息

Kaldiani Payam Mehdipour

机构信息

Department of Sciences, Naragh Branch, Islamic Azad University, Naragh, Iran; Department of Physics, West Tehran Branch, Islamic Azad University, Tehran, Iran.

出版信息

Appl Radiat Isot. 2024 Oct;212:111464. doi: 10.1016/j.apradiso.2024.111464. Epub 2024 Aug 3.

Abstract

The fission fragment total excitation energy, TXE(A), is investigated for neutron-induced fission of uranium isotopes using three different methods. Different methods for calculations of the TXE(A) produced by the decay of low excited systems are analyzed and their results are compared with the available TXE values. The calculated TXE values have been compared with the results of other studies for the neutron induced fission of U, U as well as the photo-fission of U. The scission point method for evaluating TXE has been modified by comparing the available and calculated results. TXE(A) is evaluated for other uranium isotopes using three methods. It is found that TXE values in the neutron induced fission of U, U and the photo-fission of U are greater than the calculated TXE values of other uranium isotopes. The TXE values of light uranium isotopes decrease with increasing their mass numbers, while the TXE values of heavy uranium isotopes increase as their mass numbers increase. Also, the calculated TXE values for all isotopes increase sharply near the symmetric region, which is due to the formation of unstable fission fragment. On the other hand, a slight increase in neutron multiplicity and TXE values can be observed in heavy fission fragments (A>155), which could be due to the neutron excess. However, the sharp increase in neutron multiplicity and TXE values in some studies for the heavy fission fragments (A>155) is due to a missing correction in the data analysis.

摘要

利用三种不同方法研究了铀同位素中子诱发裂变的裂变碎片总激发能TXE(A)。分析了计算低激发系统衰变产生的TXE(A)的不同方法,并将其结果与现有的TXE值进行了比较。将计算得到的TXE值与其他关于U、U的中子诱发裂变以及U的光致裂变的研究结果进行了比较。通过比较现有结果和计算结果,对评估TXE的断列点方法进行了修正。使用三种方法评估了其他铀同位素的TXE(A)。发现U、U的中子诱发裂变以及U的光致裂变中的TXE值大于其他铀同位素的计算TXE值。轻铀同位素的TXE值随质量数增加而降低,而重铀同位素的TXE值随质量数增加而增加。此外,所有同位素的计算TXE值在对称区域附近急剧增加,这是由于不稳定裂变碎片的形成。另一方面,在重裂变碎片(A>155)中可以观察到中子多重性和TXE值略有增加,这可能是由于中子过剩。然而,一些关于重裂变碎片(A>155)的研究中中子多重性和TXE值的急剧增加是由于数据分析中缺少校正。

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