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化学活性胶体或酶液滴中的异常波动。

Anomalous Fluctuations in a Droplet of Chemically Active Colloids or Enzymes.

作者信息

Prathyusha K R, Saha Suropriya, Golestanian Ramin

机构信息

<a href="https://ror.org/0087djs12">Max Planck Institute for Dynamics and Self-Organization (MPI-DS)</a>, D-37077 Göttingen, Germany.

<a href="https://ror.org/01bf9rw71">Max Planck Institute for Physics of Complex Systems</a>, Dresden, Germany.

出版信息

Phys Rev Lett. 2024 Aug 2;133(5):058401. doi: 10.1103/PhysRevLett.133.058401.

Abstract

Chemically active colloids or enzymes cluster into dense droplets driven by their phoretic response to collectively generated chemical gradients. Employing Brownian dynamics simulation techniques, our study of the dynamics of such a chemically active droplet uncovers a rich variety of structures and dynamical properties, including the full range of fluidlike to solidlike behavior, and non-Gaussian positional fluctuations. Our work sheds light on the complex dynamics of the active constituents of metabolic clusters, which are the main drivers of nonequilibrium activity in living systems.

摘要

化学活性胶体或酶会因它们对共同产生的化学梯度的泳动响应而聚集形成致密液滴。利用布朗动力学模拟技术,我们对这种化学活性液滴动力学的研究揭示了丰富多样的结构和动力学特性,包括从完全类似流体到类似固体的行为范围,以及非高斯位置涨落。我们的工作揭示了代谢簇活性成分的复杂动力学,而代谢簇是生命系统中非平衡活动的主要驱动因素。

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