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Kagome晶格中本征对称性破缺自旋纹理的实空间成像

Real-Space Imaging of Intrinsic Symmetry-Breaking Spin Textures in a Kagome Lattice.

作者信息

Xie Caihong, Deng Yongcheng, Zhang Dong, Li Junbo, Xiong Yimin, Ma Mangyuan, Ma Fusheng, Tong Wei, Wang Jihao, Meng Wenjie, Hou Yubin, Han Yuyan, Feng Qiyuan, Lu Qingyou

机构信息

University of Science and Technology of China, Hefei, 230026, China.

Anhui Province Key Laboratory of Low-Energy Quantum Materials and Devices, High Magnetic Field Laboratory, HFIPS, Chinese Academy of Sciences, Hefei, 230031, China.

出版信息

Adv Sci (Weinh). 2024 Oct;11(39):e2404088. doi: 10.1002/advs.202404088. Epub 2024 Aug 19.

Abstract

The electronic orders in kagome materials have emerged as a fertile platform for studying exotic quantum states, and their intertwining with the unique kagome lattice geometry remains elusive. While various unconventional charge orders with broken symmetry is observed, the influence of kagome symmetry on magnetic order has so far not been directly observed. Here, using a high-resolution magnetic force microscopy, it is, for the first time, observed a new lattice form of noncollinear spin textures in the kagome ferromagnet in zero magnetic field. Under the influence of the sixfold rotational symmetry of the kagome lattice, the spin textures are hexagonal in shape and can further form a honeycomb lattice structure. Subsequent thermal cycling measurements reveal that these spin textures transform into a non-uniform in-plane ferromagnetic ground state at low temperatures and can fully rebuild at elevated temperatures, showing a strong second-order phase transition feature. Moreover, some out-of-plane magnetic moments persist at low temperatures, supporting the Kane-Mele scenario in explaining the emergence of the Dirac gap. The observations establish that the electronic properties, including both charge and spin orders, are strongly coupled with the kagome lattices.

摘要

Kagome 材料中的电子序已成为研究奇异量子态的一个富有成果的平台,但其与独特的 Kagome 晶格几何结构的交织情况仍不明确。虽然观察到了各种具有对称性破缺的非常规电荷序,但到目前为止,尚未直接观察到 Kagome 对称性对磁序的影响。在此,利用高分辨率磁力显微镜,首次在零磁场下的 Kagome 铁磁体中观察到一种非共线自旋纹理的新晶格形式。在 Kagome 晶格的六重旋转对称性影响下,自旋纹理呈六边形,并且可以进一步形成蜂窝晶格结构。随后的热循环测量表明,这些自旋纹理在低温下转变为非均匀的面内铁磁基态,在高温下可以完全重建,呈现出强烈的二级相变特征。此外,一些面外磁矩在低温下持续存在,这支持了 Kane-Mele 模型对狄拉克能隙出现的解释。这些观察结果表明,包括电荷序和自旋序在内的电子性质与 Kagome 晶格强烈耦合。

https://cdn.ncbi.nlm.nih.gov/pmc/blobs/d0ad/11497059/91e0f8329b78/ADVS-11-2404088-g001.jpg

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