Cui Songbin, Jiang Chengxin, Zhan Zhen, Wilson Ty, Zhang Naipeng, Xie Xiaoming, Yuan Shengjun, Wang Haomin, Lewandowski Cyprian, Ni Guangxin
Department of Physics, Florida State University, Tallahassee, Florida 32306, United States.
National High Magnetic Field Laboratory, Tallahassee, Florida 32310, United States.
Nano Lett. 2024 Sep 18;24(37):11490-11496. doi: 10.1021/acs.nanolett.4c02841. Epub 2024 Sep 3.
A central paradigm of moiré materials relies on the formation of superlattices that yield enlarged effective crystal unit cells. While a critical consequence of this phenomenon is the celebrated flat electronic bands that foster strong interaction effects, the presence of superlattices has further implications. Here we explore the advantages of moiré superlattices in twisted bilayer graphene (TBG) aligned with hexagonal boron nitride (hBN) for passively enhancing optical conductivity in the low-energy regime. To probe the local optical response of TBG/hBN double-moiré lattices, we use infrared (IR) nano-imaging in conjunction with nanocurrent imaging to examine local optical conductivity over a wide range of TBG twist angles. We show that interband transitions associated with the multiple moiré flat and dispersive bands produce tunable transparent IR responses even at finite carrier densities, which is in stark contrast to the previously limited metallic near transparency observed only in undoped pristine graphene.
莫尔材料的一个核心范式依赖于超晶格的形成,这些超晶格会产生扩大的有效晶体单胞。虽然这一现象的一个关键结果是著名的平坦电子能带,它促进了强相互作用效应,但超晶格的存在还有其他影响。在这里,我们探索了与六方氮化硼(hBN)对齐的扭曲双层石墨烯(TBG)中的莫尔超晶格在低能区被动增强光导率的优势。为了探测TBG/hBN双莫尔晶格的局部光学响应,我们结合纳米电流成像使用红外(IR)纳米成像来检查在广泛的TBG扭曲角范围内的局部光导率。我们表明,与多个莫尔平坦带和色散带相关的带间跃迁即使在有限载流子密度下也会产生可调谐的透明红外响应,这与之前仅在未掺杂的原始石墨烯中观察到的有限金属近透明度形成鲜明对比。