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采用水气联合调控的间歇性曝气减少垃圾填埋场的碳排放。

Intermittent aeration mitigating carbon emission from landfills with gas-water joint regulation.

机构信息

School of Civil Engineering and Architecture, Zhejiang University of Science and Technology, Hangzhou, 310023, China; Zhejiang-Singapore Joint Laboratory for Urban Renewal and Future City, Hangzhou, 310023, China.

Hangzhou Wodian Environmental Protection Technology Co., Ltd, Hangzhou, 310023, China.

出版信息

J Environ Manage. 2024 Oct;369:122347. doi: 10.1016/j.jenvman.2024.122347. Epub 2024 Sep 4.

Abstract

Landfill is a significant source of atmospheric CH and CO emissions. In this study, four landfill reactor systems were constructed to investigate the effects of different ventilation methods, including continuous aeration (20 h d) and intermittent aeration (continuous aeration for 4 h d and 2 h of aeration every 12 h, twice a day), on properties of landfilled waste and emissions of CH and CO, in comparison to a traditional landfill. Compared with continuous aeration, intermittent aeration could reduce the potential global warming effect of the CH and CO emissions, especially multiple intermittent aeration. The CH and CO emissions could be predicted by the multiple linear regression model based on the contents of carbon, sulfur and/or pH during landfill stabilization. Both intermittent and continuous aeration could enhance the methane oxidation activity of landfilled waste. The aerobic methane oxidation activity of landfilled waste reached the maximums of 50.77-73.78 μg g h after aeration for 5 or 15 d, which was higher than the anaerobic methane oxidation activity (0.45-1.27 μg g h). CO was the predominant form of organic carbon loss in the bioreactor landfills. Candidatus Methylomirabilis, Methylobacter, Methylomonas and Crenothrix were the main methane-oxidating microorganisms (MOM) in the landfills. Total, NO-N, pH and Fe were the main environmental variables influencing the MOM community, among which NO-N and pH had the significant impact on the MOM community. Partial least squares path modelling indicated that aeration modes mainly influenced the emissions of CH and CO by affecting the degradation of landfilled waste, environmental variables and microbial activities. The results would be helpful for designing aeration systems to reduce the emissions of CH and CO, and the cost during landfill stabilization.

摘要

垃圾填埋场是大气 CH 和 CO 排放的重要来源。本研究构建了四个垃圾填埋反应器系统,以研究不同通风方式(连续曝气(20 h·d)和间歇曝气(每天连续曝气 4 h,每隔 12 h 曝气 2 h,每天两次))对填埋废物特性和 CH 和 CO 排放的影响,并与传统填埋场进行了比较。与连续曝气相比,间歇曝气可以减少 CH 和 CO 排放的潜在全球变暖效应,特别是多次间歇曝气。CH 和 CO 排放可以通过基于填埋稳定过程中碳、硫和/或 pH 值的多元线性回归模型进行预测。间歇和连续曝气均可增强填埋废物的甲烷氧化活性。在曝气 5 或 15 d 后,填埋废物的好氧甲烷氧化活性达到最大,为 50.77-73.78 μg·g·h,高于厌氧甲烷氧化活性(0.45-1.27 μg·g·h)。CO 是生物反应器填埋场中有机碳损失的主要形式。Candidatus Methylomirabilis、Methylobacter、Methylomonas 和 Crenothrix 是填埋场中的主要甲烷氧化微生物(MOM)。总氮、硝态氮、pH 和 Fe 是影响 MOM 群落的主要环境变量,其中硝态氮和 pH 对 MOM 群落有显著影响。偏最小二乘路径模型表明,曝气方式主要通过影响填埋废物的降解、环境变量和微生物活性来影响 CH 和 CO 的排放。这些结果有助于设计曝气系统以减少 CH 和 CO 的排放和填埋稳定过程中的成本。

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