• 文献检索
  • 文档翻译
  • 深度研究
  • 学术资讯
  • Suppr Zotero 插件Zotero 插件
  • 邀请有礼
  • 套餐&价格
  • 历史记录
应用&插件
Suppr Zotero 插件Zotero 插件浏览器插件Mac 客户端Windows 客户端微信小程序
定价
高级版会员购买积分包购买API积分包
服务
文献检索文档翻译深度研究API 文档MCP 服务
关于我们
关于 Suppr公司介绍联系我们用户协议隐私条款
关注我们

Suppr 超能文献

核心技术专利:CN118964589B侵权必究
粤ICP备2023148730 号-1Suppr @ 2026

文献检索

告别复杂PubMed语法,用中文像聊天一样搜索,搜遍4000万医学文献。AI智能推荐,让科研检索更轻松。

立即免费搜索

文件翻译

保留排版,准确专业,支持PDF/Word/PPT等文件格式,支持 12+语言互译。

免费翻译文档

深度研究

AI帮你快速写综述,25分钟生成高质量综述,智能提取关键信息,辅助科研写作。

立即免费体验

藻酸盐衍生生物质碳-二硫化钼杂化材料:用于废水处理的垂直生长/均匀分散的二硫化钼纳米片/纳米花。

Alginate-derived biomass carbon‑molybdenum disulfide heterogeneous materials: Vertically grown/uniformly dispersed molybdenum disulfide nanosheets/nanoflowers for wastewater treatment.

机构信息

School of Textile and Material Engineering, Dalian Polytechnic University, Dalian 116034, PR China.

School of Textile and Material Engineering, Dalian Polytechnic University, Dalian 116034, PR China; State Key Laboratory of Bio-Fibers and Eco-Textiles (Qingdao University), Qingdao 266071, PR China.

出版信息

Int J Biol Macromol. 2024 Nov;279(Pt 4):135467. doi: 10.1016/j.ijbiomac.2024.135467. Epub 2024 Sep 12.

DOI:10.1016/j.ijbiomac.2024.135467
PMID:39270898
Abstract

In order to improve the dispersion of molybdenum disulfide (MoS) and enhance the performance of MoS, two alginate-derived biomass carbon-MoS (BC-MoS) composites: CMB/CMS, were prepared by introducing BC during the synthesis of MoS by hydrothermal. The effects of different gels, times and temperatures of the synthesized BC-MoS were investigated, and the adsorption capacity for methylene blue (MB), basic fuchsin (BF) and copper ions (Cu) was tested. The results indicated that the vertical growth of MoS on the BC surface could be realized when using xero-gel, while the BC and MoS were mixed uniformly when using wet-gel. Compared with MoS, the hydrophilicity and water dispersibility of BC-MoS were greatly improved, and BC-MoS had better adsorption capacity for MB/BF/Cu (99.61/86.83/60 mg/g). The adsorption mechanism exhibits that the adsorption force of BC-MoS on MB/BF is mainly based on the electrostatic force, and the adsorption on Cu comes from the electrostatic force and the Lewis soft-soft interaction. This study dramatically enriches the application of transition metal chalcogenides and provides a meaningful reference for wastewater treatment.

摘要

为了提高二硫化钼(MoS)的分散性并增强其性能,通过水热法合成 MoS 时引入生物质碳(BC),制备了两种海藻酸钠衍生的生物质碳-MoS(BC-MoS)复合材料:CMB/CMS。考察了不同凝胶、合成 BC-MoS 的时间和温度的影响,并测试了对亚甲基蓝(MB)、碱性品红(BF)和铜离子(Cu)的吸附能力。结果表明,使用干凝胶时可以实现 MoS 在 BC 表面的垂直生长,而使用湿凝胶时 BC 和 MoS 均匀混合。与 MoS 相比,BC-MoS 的亲水性和水分散性得到了极大的提高,对 MB/BF/Cu 的吸附能力也更强(99.61/86.83/60mg/g)。吸附机制表明,BC-MoS 对 MB/BF 的吸附力主要基于静电力,而对 Cu 的吸附则来自静电力和路易斯软-软相互作用。本研究极大地丰富了过渡金属硫属化合物的应用,并为废水处理提供了有意义的参考。

相似文献

1
Alginate-derived biomass carbon‑molybdenum disulfide heterogeneous materials: Vertically grown/uniformly dispersed molybdenum disulfide nanosheets/nanoflowers for wastewater treatment.藻酸盐衍生生物质碳-二硫化钼杂化材料:用于废水处理的垂直生长/均匀分散的二硫化钼纳米片/纳米花。
Int J Biol Macromol. 2024 Nov;279(Pt 4):135467. doi: 10.1016/j.ijbiomac.2024.135467. Epub 2024 Sep 12.
2
In-situ growth of zinc sulfide on the surface of alginate-based biomass carbon: A new material for removing methylene blue/basic fuchsin and copper ions.在海藻酸钠基生物质碳表面原位生长硫化锌:一种用于去除亚甲基蓝/碱性品红和铜离子的新材料。
Int J Biol Macromol. 2024 Jan;256(Pt 1):128360. doi: 10.1016/j.ijbiomac.2023.128360. Epub 2023 Nov 22.
3
Molybdenum disulfide nanoflowers - doped sodium alginate/polyvinyl alcohol porous xerogel for methylene blue and copper ion adsorption.二硫化钼纳米花掺杂的海藻酸钠/聚乙烯醇多孔气凝胶对亚甲基蓝和铜离子的吸附
Int J Biol Macromol. 2023 Dec 31;253(Pt 7):127397. doi: 10.1016/j.ijbiomac.2023.127397. Epub 2023 Oct 10.
4
Bacterial Nanocellulose/MoS Hybrid Aerogels as Bifunctional Adsorbent/Photocatalyst Membranes for Water Decontamination.细菌纳米纤维素/二硫化钼杂化气凝胶作为双功能吸附剂/光催化剂膜用于水净化。
ACS Appl Mater Interfaces. 2020 Sep 16;12(37):41627-41643. doi: 10.1021/acsami.0c14137. Epub 2020 Sep 1.
5
Biomass hydrothermal carbonization solution-assisted synthesis of intercalation-expanded core-shell structured molybdenum disulfide for efficient adsorption of Cr (VI) in electroplating wastewater treatment.生物质水热碳化溶液辅助合成插层膨胀核壳结构二硫化钼用于处理电镀废水中 Cr(VI)的高效吸附。
Bioresour Technol. 2024 Jun;401:130761. doi: 10.1016/j.biortech.2024.130761. Epub 2024 Apr 29.
6
Mutual effects behind the simultaneous removal of toxic metals and cationic dyes by interlayer-expanded MoS nanosheets.层间膨胀 MoS 纳米片同时去除有毒金属和阳离子染料的相互作用。
Environ Sci Pollut Res Int. 2019 Oct;26(30):31344-31353. doi: 10.1007/s11356-019-06277-6. Epub 2019 Aug 30.
7
Properties and adsorption mechanism of magnetic biochar modified with molybdenum disulfide for cadmium in aqueous solution.改性二硫化钼磁性生物炭对水溶液中镉的性质及吸附机理
Chemosphere. 2020 Sep;255:126995. doi: 10.1016/j.chemosphere.2020.126995. Epub 2020 May 6.
8
Adsorption toward Cu(II) and inhibitory effect on bacterial growth occurring on molybdenum disulfide-montmorillonite hydrogel surface.二硫化钼-蒙脱石水凝胶表面对 Cu(II)的吸附及其对细菌生长的抑制作用。
Chemosphere. 2020 Jun;248:126025. doi: 10.1016/j.chemosphere.2020.126025. Epub 2020 Jan 25.
9
Unique selectivity and rapid uptake of molybdenum-disulfide-functionalized MXene nanocomposite for mercury adsorption.基于二硫化钼功能化 MXene 纳米复合材料的独特选择性和快速吸附汞的性能。
Environ Res. 2020 Mar;182:109005. doi: 10.1016/j.envres.2019.109005. Epub 2019 Dec 4.
10
Mechanism of As(III) removal properties of biochar-supported molybdenum-disulfide/iron-oxide system.生物炭负载二硫化钼/氧化铁体系去除砷(III)性能的机理。
Environ Pollut. 2021 Oct 15;287:117600. doi: 10.1016/j.envpol.2021.117600. Epub 2021 Jun 16.