Koizumi Mitsuo, Ito Fumiaki, Lee Jaehong, Hironaka Kota, Takahashi Tohn, Suzuki Satoshi, Arikawa Yasunobu, Abe Yuki, Lan Zechen, Wei Tianyun, Mori Takato, Hayakawa Takehito, Yogo Akifumi
Integrated Support Center for Nuclear Nonproliferation and Nuclear Security, Japan Atomic Energy Agency (JAEA), Tokai, Ibaraki, 319-1195, Japan.
High Energy Accelerator Research Organization (KEK), 1-1 Oho, Tsukuba-shi, 305-0801, Japan.
Sci Rep. 2024 Sep 19;14(1):21916. doi: 10.1038/s41598-024-72836-8.
Laser-driven neutron sources (LDNSs) can generate strong short-pulse neutron beams, which are valuable for scientific studies and engineering applications. Neutron resonance transmission analysis (NRTA) is a nondestructive technique used for determining the areal density of each nuclide in a material sample using pulsed thermal and epithermal neutrons. Herein, we report the first successful NRTA performed using an LDNS driven by the Laser for Fast Ignition Experiment at the Institute of Laser Engineering, Osaka University. The key challenge was achieving a well-resolved resonance transmission spectrum for material analysis using an LDNS with a limited number of laser shots in the presence of strong background noise. We addressed this by employing a time-gated -glass scintillation neutron detector to measure the transmission spectra, reducing the impact of electromagnetic noise and neutron and gamma-ray flashes. Output waveforms were recorded for each laser shot and analyzed offline using a counting method. This approach yielded a spectrum with distinct resonances, which were attributed to and , as confirmed through neutron transmission simulation. The spectrum was analyzed using the least-square nuclear-resonance fitting program, REFIT, demonstrating the possibility of using an LDNS for nondestructive areal-density material characterization.
激光驱动中子源(LDNSs)能够产生强大的短脉冲中子束,这对于科学研究和工程应用具有重要价值。中子共振透射分析(NRTA)是一种无损技术,用于利用脉冲热中子和超热中子确定材料样品中各核素的面密度。在此,我们报告了首次在大阪大学激光工程研究所使用用于快速点火实验的激光驱动的LDNS成功进行的NRTA。关键挑战在于,在存在强背景噪声的情况下,使用激光发射次数有限的LDNS实现用于材料分析的分辨率良好的共振透射谱。我们通过采用时间选通的硅酸镥闪烁中子探测器来测量透射谱,减少电磁噪声以及中子和伽马射线闪光的影响,解决了这一问题。记录每次激光发射的输出波形,并使用计数方法进行离线分析。这种方法产生了具有明显共振的谱,经中子透射模拟证实,这些共振归因于镅和钚。使用最小二乘核共振拟合程序REFIT对该谱进行了分析,证明了使用LDNS进行无损面密度材料表征的可能性。