Feng Xiao, Deng Ze, Guo Hongguang, Gong Li, Liu Dingrui, Feng Xiyang
College of Safety and Emergency Management Engineering, Taiyuan University of Technology, Taiyuan 030024, Shanxi, China.
Key Laboratory of In-situ Property-improving Mining of Ministry of Education, Taiyuan University of Technology, Taiyuan 030024, Shanxi, China.
Sheng Wu Gong Cheng Xue Bao. 2024 Sep 25;40(9):2884-2898. doi: 10.13345/j.cjb.240106.
Carbon capture, utilization and storage is the vital technology for China to achieve the goals of carbon peaking and carbon neutrality. Microbial activities are an indispensable part in the process of geological CO sequestration. Some microorganisms can convert CO into methane and organics as the resource for utilization or into carbonate to achieve long-term sequestration. These activities contribute to the stable storage of CO and even negative carbon emission. This paper focuses on the processes of bio-methanation, bio-liquefaction, and bio-precipitation that may be involved in CO sequestration in deep stratum and discusses the research progress in the bio-transformation pathways. Bio-methanation and bio-liquefaction can convert CO into methane or high-value organic compounds to realize resource reuse. The two technologies can be used alone or coupled to expand the application range of CO biotransformation. Bio-mineralization can convert CO into calcite by microorganism-induced carbonate precipitation, being a technology of great potential in fixing CO and limiting CO escape. At present, this field is still in the infancy stage, and there is an urgent need to establish and improve the theoretical and technical systems of CO biotransformation from transformation principle, influencing factors, conversion efficiency, economy, environmental protection, and technological conditions. Moreover, it can be combined with CCUS to establish a technical system integrating capture, transport, displace, storage, transfer, and exploit, so as to promote the value-added application of CCUS and the achievement of carbon peaking and carbon neutrality.
碳捕获、利用与封存是中国实现碳达峰和碳中和目标的关键技术。微生物活动是地质二氧化碳封存过程中不可或缺的一部分。一些微生物可以将二氧化碳转化为甲烷和有机物以供利用,或者转化为碳酸盐以实现长期封存。这些活动有助于二氧化碳的稳定封存,甚至实现负碳排放。本文重点关注深层地层二氧化碳封存可能涉及的生物甲烷化、生物液化和生物沉淀过程,并探讨生物转化途径的研究进展。生物甲烷化和生物液化可以将二氧化碳转化为甲烷或高价值有机化合物,以实现资源再利用。这两种技术可以单独使用或耦合使用,以扩大二氧化碳生物转化的应用范围。生物矿化可以通过微生物诱导碳酸盐沉淀将二氧化碳转化为方解石,这是一种在固定二氧化碳和限制二氧化碳逸出方面具有巨大潜力的技术。目前,该领域仍处于起步阶段,迫切需要从转化原理、影响因素、转化效率、经济性、环境保护和技术条件等方面建立和完善二氧化碳生物转化的理论和技术体系。此外,它可以与碳捕获、利用与封存相结合,建立一个集捕获、运输、驱替、储存、转移和开发于一体的技术体系,以促进碳捕获、利用与封存的增值应用以及碳达峰和碳中和目标的实现。