Huang Jia-Cai, Han Tian-Yang, Zhang Jie, Ni Ming-Jiu
School of Aerospace Engineering, Xi'an Jiaotong University, Xi'an 710049, China.
School of Engineering Science, University of Chinese Academy of Sciences, Beijing 100149, China.
Langmuir. 2024 Oct 8;40(40):20859-20871. doi: 10.1021/acs.langmuir.4c01084. Epub 2024 Sep 26.
Theoretical modeling is proposed to predict the maximum spreading of water-based ferrofluid droplets impacting upon dry surfaces influenced by a vertical magnetic field. Constructed on the principle of energy balance, this model demonstrates excellent agreement with numerical findings across various impact velocities, contact angles, and magnetic strengths. Notably, as magnetic field strength escalates, magnetic forces prevail over viscous and capillary forces, exerting a significant influence on spreading dynamics and diminishing the maximum spreading diameter of ferrofluid droplets if the impacting shape is spherical. However, for freely falling droplets, the shape becomes prolate before impacting and the promoted surface energy balances the magnetic inhibitory effect on droplet spreading, thus resulting in an almost unchanged maximum spreading diameter. By postulating complete conversion of initial kinetic energy into magnetic energy, a scaling law is derived for maximum spreading diameter under extremely high magnetic fields. Further interpolation with viscous dissipation and capillary effects enables universal rescaling under diverse impact conditions. Through comparison with numerical outcomes, the validity of our theoretical model is affirmed, establishing a balanced formula between distinct energy components for predicting maximum spreading diameter of ferrofluid droplets accurately.
提出了理论模型来预测受垂直磁场影响的水基铁磁流体液滴撞击干燥表面时的最大铺展情况。该模型基于能量平衡原理构建,在各种撞击速度、接触角和磁场强度下,与数值结果都表现出极好的一致性。值得注意的是,随着磁场强度的增加,磁力超过粘性力和毛细力,如果撞击形状为球形,磁力会对铺展动力学产生显著影响,并减小铁磁流体液滴的最大铺展直径。然而,对于自由下落的液滴,在撞击前形状会变为长球形,增加的表面能平衡了磁力对液滴铺展的抑制作用,从而导致最大铺展直径几乎不变。通过假设初始动能完全转化为磁能,推导出了在极高磁场下最大铺展直径的标度律。进一步考虑粘性耗散和毛细效应进行插值,可在不同撞击条件下实现通用的重新标度。通过与数值结果比较,证实了我们理论模型的有效性,建立了不同能量分量之间的平衡公式,以准确预测铁磁流体液滴的最大铺展直径。