Yao Ruizhao, Sugimoto Hiroshi, Feng Tianhua, Fujii Minoru, Liu Shimei, Li Xinming, Lan Sheng, Li Guang-Can
Guangdong Provincial Key Laboratory of Nanophotonic Functional Materials and Devices, Guangdong Basic Research Center of Excellence for Structure and Fundamental Interactions of Matter, School of Optoelectronic Science and Engineering, South China Normal University, 510006 Guangzhou, China.
Department of Electrical and Electronic Engineering, Graduate School of Engineering, Kobe University, Rokkodai Nada, Kobe 657-8501, Japan.
Nano Lett. 2024 Oct 23;24(42):13315-13323. doi: 10.1021/acs.nanolett.4c03760. Epub 2024 Oct 9.
Optical magnetic dipole (MD) emission predominantly relies on emitters with significant MD transitions, which, however, rarely exist in nature. Here, we propose a strategy to transform electric dipole (ED) emission to a magnetic one by elegantly coupling an ED emitter to a silicon nanoparticle exhibiting a strong MD resonance. This emission mode transformation enables an artificially ideal magnetic dipole source with an MD purity factor of up to 99%. The far-field emission patterns of such artificial MD sources were experimentally measured, which unambiguously resolved their magnetic-type emission origin. This study opens the path to achieving ideal magnetic dipole emission with nonmagnetic emitters, largely extending the availability of magnetic light emitters conventionally limited by nature. Beyond the fundamental significance in science, we anticipate that this study will also facilitate the development of magnetic optical nanosource and enable potential photonic applications relying on magnetic light emission.
光学磁偶极(MD)发射主要依赖于具有显著MD跃迁的发射体,然而,这种发射体在自然界中很少存在。在此,我们提出一种策略,通过巧妙地将电偶极(ED)发射体与表现出强烈MD共振的硅纳米颗粒耦合,将电偶极发射转换为磁偶极发射。这种发射模式转换能够实现一个人工理想磁偶极源,其MD纯度因子高达99%。通过实验测量了这种人工MD源的远场发射图案,明确地确定了它们的磁型发射起源。这项研究为利用非磁性发射体实现理想磁偶极发射开辟了道路,大大扩展了传统上受自然限制的磁性发光体的可用性。除了在科学上的基本意义外,我们预计这项研究还将促进磁性光学纳米源的发展,并实现依赖磁光发射的潜在光子应用。