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[中国北方五城市家庭灰尘中多溴二苯醚污染状况及影响因素分析]

[Analysis of pollution status and influencing factors of polybrominated diphenyl ethers in household dust in five cities in northern China].

作者信息

Zhang X T, Cao Y, Zhang W Y, Jiang L L, Liu M M, Song F J, Liu T T, Chen C Y, Li L, Liu H, Fan L, Du H, Sun Y M, Wang C, Luo B, Wang X L

机构信息

School of Public Health, Nanjing Medical University, Nanjing 211166, China.

China CDC Key Laboratory of Environment and Population Health, National Institute of Environmental Health, Chinese Center for Disease Control and Prevention, Beijing 100021, China.

出版信息

Zhonghua Yu Fang Yi Xue Za Zhi. 2024 Oct 6;58(10):1514-1523. doi: 10.3760/cma.j.cn112150-20231210-00422.

DOI:10.3760/cma.j.cn112150-20231210-00422
PMID:39428236
Abstract

To investigate the pollution levels and influencing factors of polybrominated diphenyl ethers (PBDEs) in household dust in five cities in northern China. Based on the "Chinese Indoor Environment and Health Surveillance" project carried out by the National Institute of Environmental Health, Chinese Center for Disease Control and Prevention in 2018-2019, during the warm season (April 2018 to September 2018) and the cold season (November 2018 to March 2019), Lanzhou in Northwest China, Shijiazhuang in North China, Panjin in Northeast China, Luoyang in Central China, and Qingdao in East China were selected as the research sites. A total of 87 families were recruited to study residences in real-life scenarios. At the same time, dust samples were collected to detect the concentration of PBDEs. The level of household environmental indicators was measured, and the residential building characteristics and family behavior habits were collected through questionnaires. A total of 142 valid dust samples and 140 valid questionnaires were obtained. The differences in PBDE concentrations across seasons, wind zones, residential building characteristics, and family habits were analyzed. The exploratory factor analysis was performed to investigate the possible sources of PBDEs, and multivariate linear regression was used to explore the factors influencing PBDEs in household dust. The ( ) of total PBDE concentrations in 142 household dust samples in five cities was 144.51 (106.61, 222.65) ng/g in the warm season and 145.10 (98.57, 180.65) ng/g in the cold season, respectively. There were seasonal differences in the concentration of ∑PBDEs in Luoyang and Shijiazhuang (<0.01). The concentration of BDE-71 was highest among PBDE homologues, followed by BDE-66 and BDE-47. Three factors were extracted by exploratory factor analysis in the warm season, and the cumulative variance contribution rate was 67.90%. The multivariate linear regression showed that the house completion less than ten years [ (95%): 0.186 (0.013, 0.359)], infrequent home cooking [ (95%):-0.342 (-0.570, -0.114)], and increased residential PM concentration [ (95%): 0.001 (0.000, 0.002)] during the warm season, as well as the house far from driveway [ (95%): 0.093 (0.013, 0.172)], house area less than 90 m [ (95%):-0.138 (-0.264, -0.013)], and lower residential xylene concentration [ (95%):-0.006 (-0.011, -0.001)] during the cold season might be related to the elevated concentrations of ∑PBDEs in household dust. The pollution of PBDEs in household dust in five northern cities is at a medium to high level. Years of house completion, frequency of cooking at home, residential PM concentration, distance from house to driveway, house area, and residential xylene concentration may influence household PBDE concentrations.

摘要

为调查中国北方五个城市家庭灰尘中多溴二苯醚(PBDEs)的污染水平及影响因素。基于中国疾病预防控制中心环境与健康相关产品安全所于2018 - 2019年开展的“中国室内环境与健康监测”项目,在暖季(2018年4月至2018年9月)和冷季(2018年11月至2019年3月),选取中国西北的兰州、华北的石家庄、东北的盘锦、华中的洛阳以及华东的青岛作为研究地点。共招募87个家庭以研究实际生活场景中的住宅。同时,采集灰尘样本以检测PBDEs的浓度。测量家庭环境指标水平,并通过问卷收集住宅建筑特征和家庭行为习惯。共获得142份有效灰尘样本和140份有效问卷。分析了PBDEs浓度在季节、风区、住宅建筑特征和家庭习惯方面的差异。进行探索性因子分析以调查PBDEs的可能来源,并使用多元线性回归探索影响家庭灰尘中PBDEs的因素。五个城市142份家庭灰尘样本中总PBDEs浓度的()在暖季分别为144.51(106.61,222.65)ng/g,在冷季为145.10(98.57,180.65)ng/g。洛阳和石家庄的∑PBDEs浓度存在季节差异(<0.01)。在PBDE同系物中,BDE - 71的浓度最高,其次是BDE - 66和BDE - 47。暖季通过探索性因子分析提取出三个因子,累积方差贡献率为67.90%。多元线性回归显示,暖季房屋建成时间少于十年[(95%):0.186(0.013,0.359)]、在家做饭频率低[(95%): - 0.342( - 0.570, - 0.114)]以及住宅PM浓度升高[(95%):0.001(0.000,0.002)],以及冷季房屋离车道远[(95%):0.093(0.013,0.172)]、房屋面积小于90平方米[(95%): - 0.138( - 0.264, - 0.013)]和住宅二甲苯浓度较低[(95%): - 0.006( - 0.011, - 0.001)]可能与家庭灰尘中∑PBDEs浓度升高有关。中国北方五个城市家庭灰尘中PBDEs的污染处于中高水平。房屋建成年份、在家做饭频率、住宅PM浓度、房屋到车道的距离、房屋面积和住宅二甲苯浓度可能影响家庭PBDEs浓度。

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