Liu Lixiang, Yang Ke, Li Liangzhong, Liu Weiwei, Yuan Haoran, Han Yongwei, Zhang Enxiang, Zheng Yuping, Jia Yajuan
State Key Laboratory of Environmental Criteria and Risk Assessment, State Environmental Protection Key Laboratory of Regional Eco-process and Function Assessment, Chinese Research Academy of Environmental Sciences, Beijing, 100012, China.
Experimental Testing Team of Jiangxi Geological Bureau, Nanchang, 330006, China.
Sci Rep. 2024 Oct 30;14(1):26172. doi: 10.1038/s41598-024-75790-7.
Sediment dredging and aeration are used as important technical measures to remediate internal loading of sediment in polluted rivers. However, previous studies have overlooked the impact of dredging and aeration on Greenhouse gases (GHGs) emission. We established three aeration rate(six different aeration intervals), one dredging treatment to investigate the effect of aeration and dredging on pollutant removals and CO, CH and NO emissions. The results indicated the pollutants and GHGs at 2.4, 3.4, 4.4 L min aeration rates reached collaborative emission reduction after more than 3 h or within 1.5 h. Meanwhile, the GHGs fluxes after aeration decreased with the increasing aeration rate, with the mean CO, CH and NO fluxes of 69.74, 0.16, 7.53 mg m h and 33.64, 0.09, 4.17 mg m h before and after aeration, respectively. With respect to dredging, the pollutants and NO reached synergic effects between reduction of pollution and carbon emissions after 1 h dredging. Specifically, the CO and CH emissions after dredging was lower than those of before dredging, but the NO emissions was higher than those of before dredging. In addition, our analysis revealed that the dissolved oxygen (DO), oxidation-reduction potential (ORP), available potassium (AK) and ammoniacal nitrogen (NH-N) in the sediment influenced GHGs fluxes at the water-air interface in the aeration. Our study indicated moderate aeration and dredging can achieve the synergistic effect in reducing pollution and carbon emissions.
底泥疏浚和曝气是修复污染河流底泥内源污染的重要技术措施。然而,以往的研究忽略了疏浚和曝气对温室气体(GHGs)排放的影响。我们设置了三种曝气速率(六种不同曝气间隔)和一种疏浚处理,以研究曝气和疏浚对污染物去除及CO₂、CH₄和N₂O排放的影响。结果表明,在曝气速率为2.4、3.4、4.4 L·min时,污染物和温室气体在曝气3 h以上或1.5 h内达到协同减排效果。同时,曝气后温室气体通量随曝气速率的增加而降低,曝气前后CO₂、CH₄和N₂O的平均通量分别为69.74、0.16、7.53 mg·m⁻²·h⁻¹和33.64、0.09、4.17 mg·m⁻²·h⁻¹。对于疏浚,疏浚1 h后污染物和N₂O在污染减排和碳排放之间达到协同效应。具体而言,疏浚后CO₂和CH₄排放低于疏浚前,但N₂O排放高于疏浚前。此外,我们的分析表明,底泥中的溶解氧(DO)、氧化还原电位(ORP)、速效钾(AK)和氨氮(NH₃-N)影响曝气过程中水-气界面的温室气体通量。我们的研究表明,适度的曝气和疏浚可以在减少污染和碳排放方面实现协同效应。