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用于安全核退役的激光切割中的二次发射行为分析和气溶胶特性评估。

Secondary emission behavior analysis and aerosol characteristics evaluation in laser cutting for safe nuclear decommissioning.

作者信息

Ock Joonsoo, Shin Jae Sung, Lim Gwon, Song Ki-Hee, Oh Seong Y, Yang Wonseok, Choi Sungyeol

机构信息

Department of Nuclear Engineering, Seoul National University, 1 Gwanak-ro, Gwanak-gu, Seoul 08826, Republic of Korea.

Quantum Optics Research Division, Korea Atomic Energy Research Institute, 111 Daedeok-daero 989beon-gil, Yuseong-gu, Daejeon 34057, Republic of Korea; Department of Radiation Science, University of Science and Technology, 217 Gajeong-ro, Yuseong-gu, Daejeon 34113, Republic of Korea.

出版信息

J Hazard Mater. 2024 Dec 5;480:136274. doi: 10.1016/j.jhazmat.2024.136274. Epub 2024 Oct 28.

Abstract

We analyzed secondary emissions and aerosol characteristics generated during the cutting of 10-30 mm thick austenitic 304 L stainless-steel plates with a high-power fiber laser. This study comprehensively includes exhausted aerosols, sedimented dross, wall deposits, and attached slag. The amount of secondary emissions for each cutting process condition was determined by type. Over 98 % of the secondary emissions consisted of attached slag and sedimented dross, with wall deposits accounting for 0.5-1.4 % and exhausted aerosols for less than 0.1 %. As cutting thickness increased, the total amount of secondary emissions increased. The ratios of attached slag and sedimented dross varied depending on cutting speed and laser power. The count median aerodynamic diameter of aerosols was ∼0.12 µm when a 30 mm thick plate was cut with a laser power of 3 kW. Aerosol concentration decreased by nearly 30 % with increasing cutting speed, depending on conditions, suggesting that optimizing speeds can effectively reduce aerosol generation. Chemical composition analysis provides insights into aerosol reactivity, toxicity, and environmental impacts, aiding in the design of filtration and ventilation systems. These results are expected to reduce environmental and health impacts in nuclear decommissioning processes.

摘要

我们分析了用高功率光纤激光切割10 - 30毫米厚的奥氏体304L不锈钢板时产生的二次排放物和气溶胶特性。本研究全面涵盖了排放的气溶胶、沉积的熔渣、壁面沉积物和附着的炉渣。针对每种切割工艺条件,按类型确定二次排放物的量。超过98%的二次排放物由附着的炉渣和沉积的熔渣组成,壁面沉积物占0.5 - 1.4%,排放的气溶胶占比不到0.1%。随着切割厚度增加,二次排放物总量增加。附着炉渣和沉积熔渣的比例随切割速度和激光功率而变化。当用3千瓦激光功率切割30毫米厚的板材时,气溶胶的计数中值空气动力学直径约为0.12微米。根据条件不同,随着切割速度增加,气溶胶浓度降低近30%,这表明优化速度可有效减少气溶胶生成。化学成分分析有助于了解气溶胶的反应性、毒性和环境影响,有助于设计过滤和通风系统。这些结果有望减少核退役过程中的环境和健康影响。

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