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使用具有偏振可区分发射光谱的双脊超表面发射器进行高灵敏度多气体检测。

High-sensitivity multi-gas detection using dual-ridge metasurface emitters with polarization-distinguishable emission spectra.

作者信息

Song Feng, Wu Xiaohu, Liu Yufang, Yu Kun

出版信息

Opt Express. 2024 Nov 4;32(23):41244-41254. doi: 10.1364/OE.541087.

Abstract

The metasurface thermal emitter offers an energy-efficient, compact, and sensitive solution as a radiation source for non-contact gas detection, enabling the "molecular fingerprint" technique to be widely applied, from medical diagnostics to environmental monitoring. However, most narrowband emitters are designed for a single target gas, hindering the miniaturization of multi-gas detection systems. In this work, a one-dimensional dual-ridge grating emitter is employed, achieving dual-band and tri-band polarization-distinguishable emission spectra through the excitation of Fabry-Perot (FP) resonances and quasi-bound states in the continuum (qBICs). These emission spectra can be readily matched to multiple non-overlapping absorption peaks of gases such as CH, CO, CO, NO, and NH within the 3-6 µm range, thereby reducing the impact of mixed gases on measurements. Compared to conventional metal-dielectric-metal structures, the use of a single metal layer results in lower material losses, enabling higher Q-factors and more pronounced directional radiation intensity variations. Furthermore, adjusting the asymmetry to modulate the qBIC-excited absorption peaks does not affect the Q-factor of the FP resonance absorption, thus achieving high-sensitivity multi-band gas detection. This work provides a promising approach for the miniaturization and integration of multi-gas channel detection, facilitating more accurate and sensitive sensing strategies.

摘要

超表面热发射器作为一种用于非接触式气体检测的辐射源,提供了一种节能、紧凑且灵敏的解决方案,使“分子指纹”技术能够从医学诊断到环境监测等领域得到广泛应用。然而,大多数窄带发射器是为单一目标气体设计的,这阻碍了多气体检测系统的小型化。在这项工作中,采用了一维双脊光栅发射器,通过激发法布里 - 珀罗(FP)共振和连续谱中的准束缚态(qBICs)实现了双波段和三波段偏振可区分的发射光谱。这些发射光谱可以很容易地与3 - 6微米范围内的CH、CO、CO、NO和NH等气体的多个不重叠吸收峰相匹配,从而减少混合气体对测量的影响。与传统的金属 - 介质 - 金属结构相比,使用单一金属层可降低材料损耗,实现更高的品质因数和更明显的定向辐射强度变化。此外,调整不对称性以调制qBIC激发的吸收峰不会影响FP共振吸收的品质因数,从而实现高灵敏度多波段气体检测。这项工作为多气体通道检测的小型化和集成提供了一种有前景的方法,有助于实现更准确、灵敏的传感策略。

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