Lin Chun, Consiglio Armando, Forslund Ola Kenji, Küspert Julia, Denner M Michael, Lei Hechang, Louat Alex, Watson Matthew D, Kim Timur K, Cacho Cephise, Carbone Dina, Leandersson Mats, Polley Craig, Balasubramanian Thiagarajan, Sante Domenico Di, Thomale Ronny, Guguchia Zurab, Sangiovanni Giorgio, Neupert Titus, Chang Johan
Physik-Institut, Universität Zürich, Zürich, Switzerland.
Stanford Synchrotron Radiation Lightsource, SLAC National Accelerator Laboratory, Menlo Park, USA.
Nat Commun. 2024 Dec 2;15(1):10466. doi: 10.1038/s41467-024-53737-w.
Tunable quantum materials hold great potential for applications. Of special interest are materials in which small lattice strain induces giant electronic responses. The kagome compounds AVSb (A = K, Rb, Cs) provide a testbed for electronic tunable states. In this study, through angle-resolved photoemission spectroscopy, we provide comprehensive spectroscopic measurements of the electronic responses induced by compressive and tensile strains on the charge-density-wave (CDW) and van Hove singularity (VHS) in CsVSb. We observe a tripling of the CDW gap magnitudes with ~ 1% strain. Simultaneously, changes of both energy and mass of the VHS are observed. Combined, this reveals an anticorrelation between the unconventional CDW order parameter and the mass of the VHS, and highlight the role of the latter in the superconducting pairing. The substantial electronic responses uncover a rich strain tunability of the versatile kagome system in studying quantum interplays under lattice variations.
可调谐量子材料具有巨大的应用潜力。特别令人感兴趣的是那些小晶格应变能引发巨大电子响应的材料。 Kagome化合物AVSb(A = K、Rb、Cs)为电子可调谐态提供了一个试验平台。在本研究中,通过角分辨光电子能谱,我们对CsVSb中由压缩应变和拉伸应变在电荷密度波(CDW)和范霍夫奇点(VHS)上引发的电子响应进行了全面的光谱测量。我们观察到,在约1%的应变下,CDW能隙大小增加了两倍。同时,还观察到VHS的能量和质量都发生了变化。综合来看,这揭示了非常规CDW序参量与VHS质量之间的反相关性,并突出了后者在超导配对中的作用。这些显著的电子响应揭示了多功能Kagome系统在研究晶格变化下的量子相互作用时具有丰富的应变可调谐性。